Water vapour and CO2 fluxes were measured by the eddy-covariance technique above a mixed needle and broad-leaved forest with affiliated meteorological measurements in Changbai Mountain as part of China's FLUX proj...Water vapour and CO2 fluxes were measured by the eddy-covariance technique above a mixed needle and broad-leaved forest with affiliated meteorological measurements in Changbai Mountain as part of China's FLUX projects since late August in 2002. Net water vapour exchange and environmental control over the forest were examined from September 1 to October 31 in 2002. To quantify the seasonal dynamics, the transition period was separated into leafed, leaf falling and leafless stages according to the development of leaf area. The results showed that (a) seasonal variation of water vapour exchange was mainly controlled by net radiation (Rn) which could account for 78.5%, 63.4% and 56.6% for leafed, leaf falling and leafless stages, respectively, while other environmental factors' effects varied evidently; (b) magnitude of water vapour flux decreased remarkably during autumn and daily mean of water vapour exchange was 24.2 mg m-2 s-1 (100%), 14.8 mg m-2 s-1 (61.2%) and 10.3 mg m-2 s-1 (42.6%) for leafed, leaf falling and leafless stage, respectively; and (c) the budget of water vapour exchange during autumn was estimated to be 87.1 kg H2O m-2, with a mean of 1427.2 g H2O d-1' varying markedly from 3104.0 to 227.5 g H2O m-2d-1.展开更多
Global Positioning System （GPS） has been widely used to estimate the total zenith tropo- spheric delay （ZTD） and precipitable water vapour （PWV） for weather prediction and at- mospheric research as a continuous ...Global Positioning System （GPS） has been widely used to estimate the total zenith tropo- spheric delay （ZTD） and precipitable water vapour （PWV） for weather prediction and at- mospheric research as a continuous and all-weather technique. However, estimations of ZTD and PWV are subject to effects of geophysical models with large uncertainties, particularly imprecise ocean tide models of inland seas in Turkey. In this paper, GPS data from Jan. 1, 2010 to Dec. 31, 2011 are processed using GAMIT/GLOBK at four co-located GPS stations （ISTN, ERZR, SAMN, and IZMI） with Radiosonde from the Turkish Met-Office together with several nearby IGS stations. Four widely used ocean tide models are adopted to evaluate their effects on GPS-estimated PWV, such as IERS recommended FES2004, NAO99b, CSR4.0 and GOT00. Five different strategies are taken without ocean tide model and with four ocean tide models, respectively, which are used to evaluate ocean tide models effects on GPS-estimated PWV through comparing with co-located Radiosonde. Results showed that ocean tide models have greatly affected the estimation of the pre- cipitable water vapour at stations near coasts. The ocean tide model FES2004 gave the best results when compared to Radiosonde with ＋2.12 mm in PWV at stations near coastline. While other ocean tides models agree each other at millimeter level in PWV. However, at inland GPS stations, ocean tide models have less effect on GPS-estimated PWV.展开更多
In the present work,the solubility of water vapour in tundish slag has been studied in the temperature range from 1 400 C to 1 600 C by a thermogravimetric technique.The water vapour capacity of the slags was calculat...In the present work,the solubility of water vapour in tundish slag has been studied in the temperature range from 1 400 C to 1 600 C by a thermogravimetric technique.The water vapour capacity of the slags was calculated and compared with the data from earlier studies.The results confirm that the solubility of water vapour in slags increases with increasing water vapour pressure.The relation between the two parameters obeys Sievert’s law.For slags with optical basicities from 0.5 to 0.8,a regression equation was obtained to express the relation between the water vapour capacity and optical basicity of slags.A tundish slag system with the desired properties can be designed according to the correlations between the optical basicity and various capacities of slags.展开更多
An underlying wetland surface comprises soil, water and vegetation and is sensitive to local climate change. Analysis of the degree of coupling between wetlands and the atmosphere and a quantitative assessment of how ...An underlying wetland surface comprises soil, water and vegetation and is sensitive to local climate change. Analysis of the degree of coupling between wetlands and the atmosphere and a quantitative assessment of how environmental factors influence latent heat flux have considerable scientific significance. Using data from observational tests of the Maduo Observatory of Climate and Environment of the Northwest Institute of Eco-Environment and Resource, CAS, from June 1 to August 31, 2014, this study analysed the time-varying characteristics and causes of the degree of coupling(Ω factor)between alpine wetlands underlying surface and the atmosphere and quantitatively calculated the influences of different environmental factors(solar radiation and vapour pressure deficit) on latent heat flux. The results were as follows:(1) Due to diurnal variations of solar radiation and wind speed, a trend developed where diurnal variations of the Ω factor were small in the morning and large in the evening. Due to the vegetation growing cycle, seasonal variations of the Ω factor present a reverse "U" trend. These trends are similar to the diurnal and seasonal variations of the absolute control exercised by solar radiation over latent heat flux. This conforms to the Omega Theory.(2) The values for average absolute atmospheric factor(surface factor or total) control exercised by solar radiation and water vapour pressure are 0.20(0.02 or 0.22) and 0.005(-0.07 or-0.06) W/(m2·Pa), respectively. Generally speaking, solar radiation and water vapour pressure deficit exert opposite forces on latent heat flux.(3) At the underlying alpine wetland surface, solar radiation primarily influences latent heat flux through its direct effects(atmospheric factor controls). Water vapour pressure deficit primarily influences latent heat flux through its indirect effects(surface factor controls) on changing the surface resistance.(4) The average Ω factor in the underlying alpine wetland surface is high during the vegetation growing season, with a value of 0.38, and the degree of coupling between alpine wetland surface and atmosphere system is low. The actual measurements agree with the Omega Theory. The latent heat flux is mainly influenced by solar radiation.展开更多
Stable isotopes in atmospheric water vapour are important tracers for investigating water vapour transport, mixing and phase transition. In recent years, with the rapid development of analytical techniques, research o...Stable isotopes in atmospheric water vapour are important tracers for investigating water vapour transport, mixing and phase transition. In recent years, with the rapid development of analytical techniques, research on water vapour stable isotopes has been widely conducted worldwide. In this review, we summarize basic theory and examine various methodologies employed to study stable isotopes in atmospheric water vapour, ranging from traditional collection methods to more recent advancements in laser absorption spectroscopy, satellite remote sensing, and isotope general circulation models(iGCMs). We pointed out the critical role played by isotopes in tracing moisture sources, understanding precipitation patterns, and reconstructing past climates. We identify gaps in knowledge, particularly in the representation of isotopic processes in climate models. Furthermore, we highlighted future research should focus on enhancing isotopic measurement technologies, integrating isotopic data with climatic indicators to improve model accuracy, and expanding isotopic studies to underserved water cycle dynamics. This review aims to provide suggestions for future investigations to deepen our understanding of atmospheric water vapour stable isotopes and their significance in climatology and hydrology.展开更多
Owing to the scarcity of observation data in the western Tibetan Plateau(TP),the knowledge of precipitation changes over the entire plateau based only on the limited data in eastern TP is not reliable.Therefore,the al...Owing to the scarcity of observation data in the western Tibetan Plateau(TP),the knowledge of precipitation changes over the entire plateau based only on the limited data in eastern TP is not reliable.Therefore,the alternative high-resolution precipitation data of the China Meteorological Forcing Dataset(CMFD)are used for the comprehensive analysis of precipitation changes over the whole TP(including western and northern TP)to fill in the lack of understanding of precipitation in the western TP.Compared with observations,CMFD can broadly capture the spatial distributions and identify the temporal variabilities of precipitation over the TP.Results with CMFD data suggested that the annual precipitation over the whole TP did not show a uniform humidification trend in 1979-2018 and featured wetting and drying trends in the northern(NTP)and southern TP(STP),respectively.Additionally,the four seasonal regimes of precipitation over the northern TP(NTP,including most areas of western TP)all experienced a noticeable interdecadal shift around the late 1990s,followed by above-normal precipitation.Except for spring,the seasonal precipitation over the southern TP(STP)showed interannual variations.Spring precipitation over the STP has undergone moistening since the late 1990s,which was consistent with that over the NTP.Four different reanalysis datasets,namely JRA55,MERRA2,ERA5 and CRA40,were used to compare the water vapour budget of each boundary over the TP.The increase in spring precipitation over the NTP and STP was found to be related to the decrease in water vapour outflow from the north boundary.The interdecadal increase in summer precipitation over the NTP was mainly due to the reduction of outflow from the east boundary.Finally,the increase in autumn precipitation was related to the increase in inflow from the west boundary.展开更多
Tropical cyclone(TC)-related rainfall mostly depends on the atmospheric moisture uptake from local and remote sources.In this study,the mean water vapour residence time(MWVRT)was computed for precipitation related to ...Tropical cyclone(TC)-related rainfall mostly depends on the atmospheric moisture uptake from local and remote sources.In this study,the mean water vapour residence time(MWVRT)was computed for precipitation related to TCs in each basin and on a global scale by applying a Lagrangian moisture source diagnostic method.According to our results,the highest MWVRT was found for the TCs over the South Indian Ocean and South Pacific Ocean basins(~3.08 days),followed by the Western North Pacific Ocean,Central and East North Pacific Ocean,North Indian Ocean,and North Atlantic Ocean basins(which exhibited values of 2.98,2.94,2.85,and 2.72 days,respectively).We also found a statistically significant(p<0.05)decrease in MWVRT,at a rate of~2.4 h/decade in the North Indian Ocean and~1.0 h/decade in the remaining basins.On average,the MWVRT decreased during the 24 h before TCs made landfall,and the atmospheric parcels precipitated faster after evaporation when TCs moved over land than over the ocean.Further research should focus on the relationship between global warming and MWVRT of atmospheric parcels that precipitate over TC positions.展开更多
Soil-water characteristics of Gaomiaozi(GMZ)Ca-bentonite at high suctions(3–287MPa)are measured by vapour equilibrium technique.The soil-water retention curve(SWRC)of samples with the same initial compaction states i...Soil-water characteristics of Gaomiaozi(GMZ)Ca-bentonite at high suctions(3–287MPa)are measured by vapour equilibrium technique.The soil-water retention curve(SWRC)of samples with the same initial compaction states is obtained in drying and wetting process.At high suctions,the hysteresis behaviour is not obvious in relationship between water content and suction,while the opposite holds between degree of saturation and suction.The suction variation can change its water retention behaviour and void ratio.Moreover,changes of void ratio can bring about changes in degree of saturation.Therefore,the total change in degree of saturation includes changes caused by suction and that by void ratio.In the space of degree of saturation and suction,the SWRC at constant void ratio shifts to the direction of higher suctions with decreasing void ratio.However,the relationship between water content and suction is less affected by changes of void ratio.The degree of saturation decreases approximately linearly with increasing void ratio at a constant suction.Moreover,the slope of the line decreases with increasing suction and they show an approximately linear relationship in semi-logarithmical scale.From this linear relationship,the variation of degree of saturation caused by the change in void ratio can be obtained.Correspondingly,SWRC at a constant void ratio can be determined from SWRC at different void ratios.展开更多
The aim of this work is an improvement of the parameterization of the soil moisture in the scheme of the Land Surface Process Model (LSPM) for applications over desert areas. In fact, in very dry conditions, the water...The aim of this work is an improvement of the parameterization of the soil moisture in the scheme of the Land Surface Process Model (LSPM) for applications over desert areas. In fact, in very dry conditions, the water vapour flux plays an important role in the evaporation processes and influences the underground profiles of humidity and temperature. The improved version of soil moisture parameterization in the LSPM scheme has been checked by using the data taken from the database of the field experiment HAPEX-Sahel (Hydrology-Atmosphere Pilot Experiment in the Sahel, 1990-1992). Model simulations refer to three dif- ferent stations located in Niger (Fallow, Millet and Tiger sites) where input data for LSPM and observations were simultaneously available. The results of simulations, taking into account the water vapour flux in the soil model LSPM, seem to compare better with the observed behaviour of soil moisture and turbulent heat fluxes than those overlooking the water vapour flux, confirming the great importance of the water vapour in such dry conditions.展开更多
Theory and evidence indicate that trees and other vegetation influence the atmospheric water-cycle in various ways.These influences are more important, more complex, and more poorly characterised than is widely realis...Theory and evidence indicate that trees and other vegetation influence the atmospheric water-cycle in various ways.These influences are more important, more complex, and more poorly characterised than is widely realised.While there is little doubt that changes in tree cover will impact the water-cycle, the wider consequences remain difficult to predict as the underlying relationships and processes remain poorly characterised. Nonetheless, as forests are vulnerable to human activities, these linked aspects of the water-cycle are also at risk and the potential consequences of large scale forest loss are severe. Here, for non-specialist readers, I review our knowledge of the links between vegetation-cover and climate with a focus on forests and rain(precipitation). I highlight advances, uncertainties and research opportunities. There are significant shortcomings in our understanding of the atmospheric hydrological cycle and of its representation in climate models. A better understanding of the role of vegetation and tree-cover wil reduce some of these shortcomings. I outline and il ustrate various research themes where these advances may be found.These themes include the biology of evaporation, aerosols and atmospheric motion, as well as the processes that determine monsoons and diurnal precipitation cycles. A novel theory—the ‘biotic pump’—suggests that evaporation and condensation can exert a major influence over atmospheric dynamics. This theory explains how high rainfall can be maintained within those continental land-masses that are sufficiently forested. Feedbacks within many of these processes can result in non-linear behaviours and the potential for dramatic changes as a result of forest loss(or gain): for example, switching from a wet to a dry local climate(or visa-versa). Much remains unknown and multiple research disciplines are needed to address this: forest scientists and other biologists have a major role to play.New ideas, methods and data offer opportunities to improve understanding. Expect surprises.展开更多
Boehmite was prepared under heat treatment in water vapour, and the phase transformation of gibbsite heat-treated at various temperatures was investigated. The sample was characterized by scanning electron microscopy(...Boehmite was prepared under heat treatment in water vapour, and the phase transformation of gibbsite heat-treated at various temperatures was investigated. The sample was characterized by scanning electron microscopy(SEM), X-ray diffraction (XRD), thermogravimetry and differential thermalanalysis (TG-DTA), fourier transform infrared (FTIR),and BET surface area.Effect of temperature on preparation was studied in the range of 155°–195°.With the increase in temperature, transformation of gibbsite into crystalline boehmites took place as indicated by the X-ray diffraction (XRD). The shape of the grains in the prepared sample was cube-like morphology.In water vapour gibbsite transform into boehmite by a dissolution - precipitation mechanism.展开更多
This study was aimed at gaining further insight on the role of hydration in adsorption processes of biopolymer/adsorbate systems using complementary methods (electromagnetic interference (EMI) shielding, calorimetry, ...This study was aimed at gaining further insight on the role of hydration in adsorption processes of biopolymer/adsorbate systems using complementary methods (electromagnetic interference (EMI) shielding, calorimetry, and solvent/vapour adsorption isotherms). Cellulose and starch-based materials were used as the adsorbents, whereas water (liquid and vapour), ethanol and p-nitrophenol (PNP) in aqueous solution were the adsorbate systems. The biopolymer/water systems had higher uptake capacity overall, where starch materials showed higher uptake capacity than cellulose among the various solvents. The secondary and tertiary structure of the biopolymers was a key factor affecting their uptake capacity, as evidenced by the enhanced adsorption properties of starch over cellulose, along with higher uptake of amylose (AM) versus amylopectin (AP) in starch biopolymers. EMI results also confirmed that AM starch had higher adsorption toward water than ethanol. The textural properties and surface chemistry of the biopolymers were probed using dye adsorption (PNP at pH 8.5) in aqueous solution that showed parallel trends with water vapour adsorption isotherms. Isothermal Titration Calorimetry (ITC) revealed that the heat of adsorption in AP differed from that of AM since the biopolymer tertiary structure governs the accessibility of biopolymer adsorption sites. The role of branching in AP and amorphous domains in AM/AP composites are inferred to play a key role in hydration-driven allosterism known for such biopolymer/water vapour adsorption processes.展开更多
Photosynthetic capacity for heritage (Taewa) and modern potato cultivars were compared at different water and nitrogenregimes in the glasshouse and field. The glasshouse was 2*2*4 factorial design with two irrigation:...Photosynthetic capacity for heritage (Taewa) and modern potato cultivars were compared at different water and nitrogenregimes in the glasshouse and field. The glasshouse was 2*2*4 factorial design with two irrigation: 100% ET and 60% ET;two applied N: 50 kg N ha-1 and 200 kg N ha-1, two Taewa (Moe Moe, Tutaekuri) and two modern potatoes (Moonlight, Agria). The 2009/2010 field experiment was a split-plot, with irrigation and rain-fed regimes as the main treatments: four potatoes above were sub-treatments. The 2010/2011 field experiment was a split-split-plot, with three water regimes as the main treatments: three cultivars (Moe Moe, Tutaekuri, and Agria) were subplots;two N rates were sub-sub-treatments. Gaseous exchange was measured by CIRAS-2 at different days from emergence. Leaf water potential was measured using pressure chamber method. Taewa achieved high photosynthetic WUE in glasshouse and 2010/2011 experiment by maintaining high An, low gs and low Ci compared to modern cultivars (p The An, gs and T increased with irrigation and N increase while decreasing Ci (p < 0.01). Water stress significantly increased VPD resulting in low An and photosynthetic WUE in Moonlight in the glasshouse. The leaf water potential for Taewa was very tolerant while modern potatoes were weakened by water stress. The study indicated that Taewa can be scheduled at partial irrigation without more detrimental effects on photosynthetic capacity while modern potatoes need full irrigation to avoid detrimental effects on photosynthetic capacity.展开更多
基金Knowledge Innovation Project of CAS,No.KZCX1-SW-01-01A
文摘Water vapour and CO2 fluxes were measured by the eddy-covariance technique above a mixed needle and broad-leaved forest with affiliated meteorological measurements in Changbai Mountain as part of China's FLUX projects since late August in 2002. Net water vapour exchange and environmental control over the forest were examined from September 1 to October 31 in 2002. To quantify the seasonal dynamics, the transition period was separated into leafed, leaf falling and leafless stages according to the development of leaf area. The results showed that (a) seasonal variation of water vapour exchange was mainly controlled by net radiation (Rn) which could account for 78.5%, 63.4% and 56.6% for leafed, leaf falling and leafless stages, respectively, while other environmental factors' effects varied evidently; (b) magnitude of water vapour flux decreased remarkably during autumn and daily mean of water vapour exchange was 24.2 mg m-2 s-1 (100%), 14.8 mg m-2 s-1 (61.2%) and 10.3 mg m-2 s-1 (42.6%) for leafed, leaf falling and leafless stage, respectively; and (c) the budget of water vapour exchange during autumn was estimated to be 87.1 kg H2O m-2, with a mean of 1427.2 g H2O d-1' varying markedly from 3104.0 to 227.5 g H2O m-2d-1.
文摘Global Positioning System （GPS） has been widely used to estimate the total zenith tropo- spheric delay （ZTD） and precipitable water vapour （PWV） for weather prediction and at- mospheric research as a continuous and all-weather technique. However, estimations of ZTD and PWV are subject to effects of geophysical models with large uncertainties, particularly imprecise ocean tide models of inland seas in Turkey. In this paper, GPS data from Jan. 1, 2010 to Dec. 31, 2011 are processed using GAMIT/GLOBK at four co-located GPS stations （ISTN, ERZR, SAMN, and IZMI） with Radiosonde from the Turkish Met-Office together with several nearby IGS stations. Four widely used ocean tide models are adopted to evaluate their effects on GPS-estimated PWV, such as IERS recommended FES2004, NAO99b, CSR4.0 and GOT00. Five different strategies are taken without ocean tide model and with four ocean tide models, respectively, which are used to evaluate ocean tide models effects on GPS-estimated PWV through comparing with co-located Radiosonde. Results showed that ocean tide models have greatly affected the estimation of the pre- cipitable water vapour at stations near coasts. The ocean tide model FES2004 gave the best results when compared to Radiosonde with ＋2.12 mm in PWV at stations near coastline. While other ocean tides models agree each other at millimeter level in PWV. However, at inland GPS stations, ocean tide models have less effect on GPS-estimated PWV.
文摘In the present work,the solubility of water vapour in tundish slag has been studied in the temperature range from 1 400 C to 1 600 C by a thermogravimetric technique.The water vapour capacity of the slags was calculated and compared with the data from earlier studies.The results confirm that the solubility of water vapour in slags increases with increasing water vapour pressure.The relation between the two parameters obeys Sievert’s law.For slags with optical basicities from 0.5 to 0.8,a regression equation was obtained to express the relation between the water vapour capacity and optical basicity of slags.A tundish slag system with the desired properties can be designed according to the correlations between the optical basicity and various capacities of slags.
基金supported by funding from the National Natural Science Foundation of China(Grant Nos.41530529 and 91737103)
文摘An underlying wetland surface comprises soil, water and vegetation and is sensitive to local climate change. Analysis of the degree of coupling between wetlands and the atmosphere and a quantitative assessment of how environmental factors influence latent heat flux have considerable scientific significance. Using data from observational tests of the Maduo Observatory of Climate and Environment of the Northwest Institute of Eco-Environment and Resource, CAS, from June 1 to August 31, 2014, this study analysed the time-varying characteristics and causes of the degree of coupling(Ω factor)between alpine wetlands underlying surface and the atmosphere and quantitatively calculated the influences of different environmental factors(solar radiation and vapour pressure deficit) on latent heat flux. The results were as follows:(1) Due to diurnal variations of solar radiation and wind speed, a trend developed where diurnal variations of the Ω factor were small in the morning and large in the evening. Due to the vegetation growing cycle, seasonal variations of the Ω factor present a reverse "U" trend. These trends are similar to the diurnal and seasonal variations of the absolute control exercised by solar radiation over latent heat flux. This conforms to the Omega Theory.(2) The values for average absolute atmospheric factor(surface factor or total) control exercised by solar radiation and water vapour pressure are 0.20(0.02 or 0.22) and 0.005(-0.07 or-0.06) W/(m2·Pa), respectively. Generally speaking, solar radiation and water vapour pressure deficit exert opposite forces on latent heat flux.(3) At the underlying alpine wetland surface, solar radiation primarily influences latent heat flux through its direct effects(atmospheric factor controls). Water vapour pressure deficit primarily influences latent heat flux through its indirect effects(surface factor controls) on changing the surface resistance.(4) The average Ω factor in the underlying alpine wetland surface is high during the vegetation growing season, with a value of 0.38, and the degree of coupling between alpine wetland surface and atmosphere system is low. The actual measurements agree with the Omega Theory. The latent heat flux is mainly influenced by solar radiation.
基金supported by the Second Tibetan Plateau Scientific Expedition and Research (STEP) Program (Grant No. 2019QZKK0208)the Innovation Program for Young Scholars of TPESER (Grant No. QNCX2022ZD-01)。
文摘Stable isotopes in atmospheric water vapour are important tracers for investigating water vapour transport, mixing and phase transition. In recent years, with the rapid development of analytical techniques, research on water vapour stable isotopes has been widely conducted worldwide. In this review, we summarize basic theory and examine various methodologies employed to study stable isotopes in atmospheric water vapour, ranging from traditional collection methods to more recent advancements in laser absorption spectroscopy, satellite remote sensing, and isotope general circulation models(iGCMs). We pointed out the critical role played by isotopes in tracing moisture sources, understanding precipitation patterns, and reconstructing past climates. We identify gaps in knowledge, particularly in the representation of isotopic processes in climate models. Furthermore, we highlighted future research should focus on enhancing isotopic measurement technologies, integrating isotopic data with climatic indicators to improve model accuracy, and expanding isotopic studies to underserved water cycle dynamics. This review aims to provide suggestions for future investigations to deepen our understanding of atmospheric water vapour stable isotopes and their significance in climatology and hydrology.
基金supported by the Second Tibetan Plateau Scientific Expedition and Research(STEP)programme(2019QZKK0102 and 2019QZKK0208)China Three Gorges Corporation(0704181)+1 种基金Innovation and development special project of China Meteorological Administration(CXFZ 2022J039)Key Innovation Team of China Meteorological Administration Climate Change Detection,Impact and Response(CMA2022ZD03).
文摘Owing to the scarcity of observation data in the western Tibetan Plateau(TP),the knowledge of precipitation changes over the entire plateau based only on the limited data in eastern TP is not reliable.Therefore,the alternative high-resolution precipitation data of the China Meteorological Forcing Dataset(CMFD)are used for the comprehensive analysis of precipitation changes over the whole TP(including western and northern TP)to fill in the lack of understanding of precipitation in the western TP.Compared with observations,CMFD can broadly capture the spatial distributions and identify the temporal variabilities of precipitation over the TP.Results with CMFD data suggested that the annual precipitation over the whole TP did not show a uniform humidification trend in 1979-2018 and featured wetting and drying trends in the northern(NTP)and southern TP(STP),respectively.Additionally,the four seasonal regimes of precipitation over the northern TP(NTP,including most areas of western TP)all experienced a noticeable interdecadal shift around the late 1990s,followed by above-normal precipitation.Except for spring,the seasonal precipitation over the southern TP(STP)showed interannual variations.Spring precipitation over the STP has undergone moistening since the late 1990s,which was consistent with that over the NTP.Four different reanalysis datasets,namely JRA55,MERRA2,ERA5 and CRA40,were used to compare the water vapour budget of each boundary over the TP.The increase in spring precipitation over the NTP and STP was found to be related to the decrease in water vapour outflow from the north boundary.The interdecadal increase in summer precipitation over the NTP was mainly due to the reduction of outflow from the east boundary.Finally,the increase in autumn precipitation was related to the increase in inflow from the west boundary.
基金support from the UVigo PhD grantssupport from the Xunta de Galicia(Galician Regional Government)under grant No.ED481A2020/193。
文摘Tropical cyclone(TC)-related rainfall mostly depends on the atmospheric moisture uptake from local and remote sources.In this study,the mean water vapour residence time(MWVRT)was computed for precipitation related to TCs in each basin and on a global scale by applying a Lagrangian moisture source diagnostic method.According to our results,the highest MWVRT was found for the TCs over the South Indian Ocean and South Pacific Ocean basins(~3.08 days),followed by the Western North Pacific Ocean,Central and East North Pacific Ocean,North Indian Ocean,and North Atlantic Ocean basins(which exhibited values of 2.98,2.94,2.85,and 2.72 days,respectively).We also found a statistically significant(p<0.05)decrease in MWVRT,at a rate of~2.4 h/decade in the North Indian Ocean and~1.0 h/decade in the remaining basins.On average,the MWVRT decreased during the 24 h before TCs made landfall,and the atmospheric parcels precipitated faster after evaporation when TCs moved over land than over the ocean.Further research should focus on the relationship between global warming and MWVRT of atmospheric parcels that precipitate over TC positions.
基金the National Natural Sciences Foundation of China (No. 41102163)
文摘Soil-water characteristics of Gaomiaozi(GMZ)Ca-bentonite at high suctions(3–287MPa)are measured by vapour equilibrium technique.The soil-water retention curve(SWRC)of samples with the same initial compaction states is obtained in drying and wetting process.At high suctions,the hysteresis behaviour is not obvious in relationship between water content and suction,while the opposite holds between degree of saturation and suction.The suction variation can change its water retention behaviour and void ratio.Moreover,changes of void ratio can bring about changes in degree of saturation.Therefore,the total change in degree of saturation includes changes caused by suction and that by void ratio.In the space of degree of saturation and suction,the SWRC at constant void ratio shifts to the direction of higher suctions with decreasing void ratio.However,the relationship between water content and suction is less affected by changes of void ratio.The degree of saturation decreases approximately linearly with increasing void ratio at a constant suction.Moreover,the slope of the line decreases with increasing suction and they show an approximately linear relationship in semi-logarithmical scale.From this linear relationship,the variation of degree of saturation caused by the change in void ratio can be obtained.Correspondingly,SWRC at a constant void ratio can be determined from SWRC at different void ratios.
文摘The aim of this work is an improvement of the parameterization of the soil moisture in the scheme of the Land Surface Process Model (LSPM) for applications over desert areas. In fact, in very dry conditions, the water vapour flux plays an important role in the evaporation processes and influences the underground profiles of humidity and temperature. The improved version of soil moisture parameterization in the LSPM scheme has been checked by using the data taken from the database of the field experiment HAPEX-Sahel (Hydrology-Atmosphere Pilot Experiment in the Sahel, 1990-1992). Model simulations refer to three dif- ferent stations located in Niger (Fallow, Millet and Tiger sites) where input data for LSPM and observations were simultaneously available. The results of simulations, taking into account the water vapour flux in the soil model LSPM, seem to compare better with the observed behaviour of soil moisture and turbulent heat fluxes than those overlooking the water vapour flux, confirming the great importance of the water vapour in such dry conditions.
基金the value of participation in the Australian Research Council projects under grants DP160102107 and LP130100498benefitted from the meeting in Leuven,Belgium in 2015 where his participation was funded by We Forest and the Center for International Forest Researchfrom the meeting in Wageningen,Netherlands,also in 2015,where his participation was funded by Tropenbos
文摘Theory and evidence indicate that trees and other vegetation influence the atmospheric water-cycle in various ways.These influences are more important, more complex, and more poorly characterised than is widely realised.While there is little doubt that changes in tree cover will impact the water-cycle, the wider consequences remain difficult to predict as the underlying relationships and processes remain poorly characterised. Nonetheless, as forests are vulnerable to human activities, these linked aspects of the water-cycle are also at risk and the potential consequences of large scale forest loss are severe. Here, for non-specialist readers, I review our knowledge of the links between vegetation-cover and climate with a focus on forests and rain(precipitation). I highlight advances, uncertainties and research opportunities. There are significant shortcomings in our understanding of the atmospheric hydrological cycle and of its representation in climate models. A better understanding of the role of vegetation and tree-cover wil reduce some of these shortcomings. I outline and il ustrate various research themes where these advances may be found.These themes include the biology of evaporation, aerosols and atmospheric motion, as well as the processes that determine monsoons and diurnal precipitation cycles. A novel theory—the ‘biotic pump’—suggests that evaporation and condensation can exert a major influence over atmospheric dynamics. This theory explains how high rainfall can be maintained within those continental land-masses that are sufficiently forested. Feedbacks within many of these processes can result in non-linear behaviours and the potential for dramatic changes as a result of forest loss(or gain): for example, switching from a wet to a dry local climate(or visa-versa). Much remains unknown and multiple research disciplines are needed to address this: forest scientists and other biologists have a major role to play.New ideas, methods and data offer opportunities to improve understanding. Expect surprises.
文摘Boehmite was prepared under heat treatment in water vapour, and the phase transformation of gibbsite heat-treated at various temperatures was investigated. The sample was characterized by scanning electron microscopy(SEM), X-ray diffraction (XRD), thermogravimetry and differential thermalanalysis (TG-DTA), fourier transform infrared (FTIR),and BET surface area.Effect of temperature on preparation was studied in the range of 155°–195°.With the increase in temperature, transformation of gibbsite into crystalline boehmites took place as indicated by the X-ray diffraction (XRD). The shape of the grains in the prepared sample was cube-like morphology.In water vapour gibbsite transform into boehmite by a dissolution - precipitation mechanism.
文摘This study was aimed at gaining further insight on the role of hydration in adsorption processes of biopolymer/adsorbate systems using complementary methods (electromagnetic interference (EMI) shielding, calorimetry, and solvent/vapour adsorption isotherms). Cellulose and starch-based materials were used as the adsorbents, whereas water (liquid and vapour), ethanol and p-nitrophenol (PNP) in aqueous solution were the adsorbate systems. The biopolymer/water systems had higher uptake capacity overall, where starch materials showed higher uptake capacity than cellulose among the various solvents. The secondary and tertiary structure of the biopolymers was a key factor affecting their uptake capacity, as evidenced by the enhanced adsorption properties of starch over cellulose, along with higher uptake of amylose (AM) versus amylopectin (AP) in starch biopolymers. EMI results also confirmed that AM starch had higher adsorption toward water than ethanol. The textural properties and surface chemistry of the biopolymers were probed using dye adsorption (PNP at pH 8.5) in aqueous solution that showed parallel trends with water vapour adsorption isotherms. Isothermal Titration Calorimetry (ITC) revealed that the heat of adsorption in AP differed from that of AM since the biopolymer tertiary structure governs the accessibility of biopolymer adsorption sites. The role of branching in AP and amorphous domains in AM/AP composites are inferred to play a key role in hydration-driven allosterism known for such biopolymer/water vapour adsorption processes.
文摘Photosynthetic capacity for heritage (Taewa) and modern potato cultivars were compared at different water and nitrogenregimes in the glasshouse and field. The glasshouse was 2*2*4 factorial design with two irrigation: 100% ET and 60% ET;two applied N: 50 kg N ha-1 and 200 kg N ha-1, two Taewa (Moe Moe, Tutaekuri) and two modern potatoes (Moonlight, Agria). The 2009/2010 field experiment was a split-plot, with irrigation and rain-fed regimes as the main treatments: four potatoes above were sub-treatments. The 2010/2011 field experiment was a split-split-plot, with three water regimes as the main treatments: three cultivars (Moe Moe, Tutaekuri, and Agria) were subplots;two N rates were sub-sub-treatments. Gaseous exchange was measured by CIRAS-2 at different days from emergence. Leaf water potential was measured using pressure chamber method. Taewa achieved high photosynthetic WUE in glasshouse and 2010/2011 experiment by maintaining high An, low gs and low Ci compared to modern cultivars (p The An, gs and T increased with irrigation and N increase while decreasing Ci (p < 0.01). Water stress significantly increased VPD resulting in low An and photosynthetic WUE in Moonlight in the glasshouse. The leaf water potential for Taewa was very tolerant while modern potatoes were weakened by water stress. The study indicated that Taewa can be scheduled at partial irrigation without more detrimental effects on photosynthetic capacity while modern potatoes need full irrigation to avoid detrimental effects on photosynthetic capacity.
