The gyroresonant interaction between electromagnetic ion cyclotron （EMIC） waves and energetic particles was studied in a multi-ion （H^＋, He^＋, and O^＋） plasma. The minimum resonant energy Emin, resonant wave fr...The gyroresonant interaction between electromagnetic ion cyclotron （EMIC） waves and energetic particles was studied in a multi-ion （H^＋, He^＋, and O^＋） plasma. The minimum resonant energy Emin, resonant wave frequency w, and pitch angle diffusion coefficient Daa were calculated at the center location of the symmetrical ring current： r ≈3.5RE with RE the Earth＇s radius. Emin is found to decrease rapidly from 10 MeV to a few keV with the increase in ca in three bands： H^＋-band, He^＋-band and O^＋-band. Moreover, EMIC waves have substantial potential to scatter energetic （～100 keV） ions （mainly H^＋ and He^＋） into the loss cone and yield precipitation loss, suggesting that wave-particle interactions contribute to ring current decay.展开更多
Head-on collisions among the single-and multi-soliton’s heavy ion acoustic waves(HIAWs) of multi-ion plasma are studied. The plasma consists of adiabatic positively charged inertial heavy ions, Boltzmann energy distr...Head-on collisions among the single-and multi-soliton’s heavy ion acoustic waves(HIAWs) of multi-ion plasma are studied. The plasma consists of adiabatic positively charged inertial heavy ions, Boltzmann energy distributed light ions and kappa energy distributed electrons. The extended poincaré-Lighthill-Kuo(e PLK) method is applied for the derivation of two-sided Korteweg–de Vries(KdV) equations(KdVEs). The KdV single-soliton solutions(KdVSSs) are determined using the hyperbolic secant method and the KdV multi-soliton solutions(KdVMSs)are obtained using the Hirota method. The effects of superthermality of electrons, temperature ratios of electron to light ion and heavy ion to electron, and the density ratio of electron to heavy ion on phase shifts are investigated for the head-on collisions between two-soliton HIAWs. The effects of plasma parameters on angular frequency, phase speed, production of multi-soliton structures, and the head-on collisions among single-, double-, triple-, quadruple-, and quintuplesolitons are also studied.展开更多
We propose a scheme for generating multi-ion graph states using many trapped ions in thermal motion.Our generation scheme is insensitive to external state since the interaction between ions and laser fields does not i...We propose a scheme for generating multi-ion graph states using many trapped ions in thermal motion.Our generation scheme is insensitive to external state since the interaction between ions and laser fields does not involvethe external degree of freedom.The scheme can be well realized within the current experimental technique.展开更多
The nonlinear propagation of the DIA (dust ion-acoustic) waves in multi-ion dense plasma system containing degener- ate electrons, both positive and negative ions, arbitrary charged dust grains has been investigated b...The nonlinear propagation of the DIA (dust ion-acoustic) waves in multi-ion dense plasma system containing degener- ate electrons, both positive and negative ions, arbitrary charged dust grains has been investigated by employing the reductive perturbation method. The nonlinear waves (solitary and shock waves) have been observed to be formed in case of both positive and negative charged dust grains from the stationary solution of the Korteweg de-Vries (K-dV) equation and Burger’s equation. The fundamental properties of such nonlinear waves have been theoretically analyzed by comparing system potential for both positive and negative dust grains. It has been shown that the basic features of these waves are significantly modified by the positive and negative ions drift speed and polarities of dust grains. The implications of our results in space and laboratory plasmas are briefly discussed.展开更多
锂离子电池健康状态(state of health,SOH)估计对确保能量存储系统的可靠性和安全性至关重要。然而,现有SOH估计方法在单一特征提取和固定充放电条件依赖方面存在局限性,难以适应多变的实际工作环境。为解决这一问题,本工作提出了一种...锂离子电池健康状态(state of health,SOH)估计对确保能量存储系统的可靠性和安全性至关重要。然而,现有SOH估计方法在单一特征提取和固定充放电条件依赖方面存在局限性,难以适应多变的实际工作环境。为解决这一问题,本工作提出了一种基于弛豫电压的并行多尺度特征融合卷积模型(multi-scale feature fusion convolution model,MSFFCM)结合极端梯度提升树(XGBoost)的SOH估计方法。MSFFCM通过多层堆叠卷积模块提取弛豫电压数据的深层特征,同时利用并行多尺度注意力机制增强了多尺度特征的捕捉能力,并将这些特征与统计特征进行融合,以提升模型的特征提取和融合能力。针对XGBoost模型,本工作应用贝叶斯优化算法进行参数调优,从而在多源融合特征基础上实现高精度SOH估计。实验验证基于两种商用18650型号电池的多温度和多充放电策略数据集,结果表明该方法的均方根误差(RMSE)和平均绝对误差(MAE)均小于0.5%,明显优于传统方法。本工作为锂电池健康管理提供了一种不依赖特定充放电条件的有效估计工具,有望在复杂的实际应用中发挥重要作用。展开更多
Aqueous rechargeable batteries using abundant multi-ion cations have receivedincreasing attention in the energy storage field for their high safety and low cost.Layered double hydroxides(LDHs)possess a two-dimensional...Aqueous rechargeable batteries using abundant multi-ion cations have receivedincreasing attention in the energy storage field for their high safety and low cost.Layered double hydroxides(LDHs)possess a two-dimensional structure andexhibit great potential as cathodes for multi-ion intercalation.However,theinsufficient active sites of LDHs result in low capacities in the discharging process.Interestingly,the LDHs after the deprotonation process exhibit favorable electrochemicalperformance of multi-cation intercalation.The deprotonation process ofLDHs has been widely found in the oxygen evolution reaction and energy storagefield,where LDHs lose H in laminates and converts to deprotonatedγ-phaseMOOHs(MOOs).Herein,we take a comprehensive overview of the dynamicsstructure transformation of the deprotonation process of LDHs.Furthermore,thedevelopment of advanced aqueous battery cathode and metal battery anode basedon deprotonated LDHs for energy storage is explored and summarized.Finally,theperspective of deprotonated LDHs in the energy storage field is discussed.展开更多
Modern medicine is increasingly interested in advanced sensors to detect and analyze biochemical indicators.Ion sensors based on potentiometric methods are a promising platform for monitoring physiological ions in bio...Modern medicine is increasingly interested in advanced sensors to detect and analyze biochemical indicators.Ion sensors based on potentiometric methods are a promising platform for monitoring physiological ions in biological subjects.Current semi-implantable devices are mainly based on single-parameter detection.Miniaturized semi-implantable electrodes for multiparameter sensing have more restrictions on the electrode size due to biocompatibility considerations,but reducing the electrode surface area could potentially limit electrode sensitivity.This study developed a semi-implantable device system comprising a multiplexed microfilament electrode cluster(MMEC)and a printed circuit board for real-time monitoring of intra-tissue K^(+),Ca^(2+),and Na^(+)concentrations.The electrode surface area was less important for the potentiometric sensing mechanism,suggesting the feasibility of using a tiny fiber-like electrode for potentiometric sensing.The MMEC device exhibited a broad linear response(K^(+):2–32 mmol/L;Ca^(2+):0.5–4 mmol/L;Na^(+):10–160 mmol/L),high sensitivity(about 20–45 mV/decade),temporal stability(>2weeks),and good selectivity(>80%)for the above ions.In vitro detection and in vivo subcutaneous and brain experiment results showed that the MMEC system exhibits good multi-ion monitoring performance in several complex environments.This work provides a platform for the continuous real-time monitoring of ion fluctuations in different situations and has implications for developing smart sensors to monitor human health.展开更多
面向电动汽车一类宽温度,大幅值、宽频率随机电流应用场景,提出一种基于全新电热耦合模型的锂电池多状态在线联合估计方法。该模型由自回归等效电路模型与单态集总热模型耦合而成,以提高模型电气动态跟随性能。电热耦合模型参数采取“...面向电动汽车一类宽温度,大幅值、宽频率随机电流应用场景,提出一种基于全新电热耦合模型的锂电池多状态在线联合估计方法。该模型由自回归等效电路模型与单态集总热模型耦合而成,以提高模型电气动态跟随性能。电热耦合模型参数采取“先验信息初始化-在线修正”的方式确定,以避免电池一致性问题带来的误差,从而实现电热耦合关系在宽温度内的连续准确表达。基于所提出的ARST(autoregression-single state thermal model)耦合模型,该文采用双滤波算法实现锂电池多状态的在线联合估计,弥补目前电池3种及以上状态联合估计的稀缺问题。最后,在[0,50]℃,基于两个动态工况,将所提出的算法与两类基于模型的多状态联合估计算法进行比较。结果表明:ARST模型具有更好的电气跟随性能;所提出的模型参数在线辨识算法能够有效提高模型精度,从而提高多状态联合估计精度;在宽温度应用中,相较仅基于电模型的多状态联合估计算法,兼顾热状态估计的多状态联合估计算法能够有效提高电池状态的估计精度。展开更多
基金National Natural Science Foundation of China (Nos.40874076,40774078,40774079 and 40536029)the Special Fund for Public Welfare Industry (meteorology)GYHY200806072the Visiting Scholar Foundation of State Key Laboratory for Space Weather,Chinese Academy of Sciences
文摘The gyroresonant interaction between electromagnetic ion cyclotron （EMIC） waves and energetic particles was studied in a multi-ion （H^＋, He^＋, and O^＋） plasma. The minimum resonant energy Emin, resonant wave frequency w, and pitch angle diffusion coefficient Daa were calculated at the center location of the symmetrical ring current： r ≈3.5RE with RE the Earth＇s radius. Emin is found to decrease rapidly from 10 MeV to a few keV with the increase in ca in three bands： H^＋-band, He^＋-band and O^＋-band. Moreover, EMIC waves have substantial potential to scatter energetic （～100 keV） ions （mainly H^＋ and He^＋） into the loss cone and yield precipitation loss, suggesting that wave-particle interactions contribute to ring current decay.
文摘Head-on collisions among the single-and multi-soliton’s heavy ion acoustic waves(HIAWs) of multi-ion plasma are studied. The plasma consists of adiabatic positively charged inertial heavy ions, Boltzmann energy distributed light ions and kappa energy distributed electrons. The extended poincaré-Lighthill-Kuo(e PLK) method is applied for the derivation of two-sided Korteweg–de Vries(KdV) equations(KdVEs). The KdV single-soliton solutions(KdVSSs) are determined using the hyperbolic secant method and the KdV multi-soliton solutions(KdVMSs)are obtained using the Hirota method. The effects of superthermality of electrons, temperature ratios of electron to light ion and heavy ion to electron, and the density ratio of electron to heavy ion on phase shifts are investigated for the head-on collisions between two-soliton HIAWs. The effects of plasma parameters on angular frequency, phase speed, production of multi-soliton structures, and the head-on collisions among single-, double-, triple-, quadruple-, and quintuplesolitons are also studied.
基金National Natural Science Foundation of China under Grant Nos.60678022 and 10704001the Specialized Research Fund for the Doctoral Program of Higher Education of Anhui Province under Grant No.20060357008+2 种基金Natural Science Foundation of Anhui Province under Grant No.070412060the Talent Foundation of Anhui UniversityAnhui Key Laboratory of Information Materials and Devices (Anhui University)
文摘We propose a scheme for generating multi-ion graph states using many trapped ions in thermal motion.Our generation scheme is insensitive to external state since the interaction between ions and laser fields does not involvethe external degree of freedom.The scheme can be well realized within the current experimental technique.
文摘The nonlinear propagation of the DIA (dust ion-acoustic) waves in multi-ion dense plasma system containing degener- ate electrons, both positive and negative ions, arbitrary charged dust grains has been investigated by employing the reductive perturbation method. The nonlinear waves (solitary and shock waves) have been observed to be formed in case of both positive and negative charged dust grains from the stationary solution of the Korteweg de-Vries (K-dV) equation and Burger’s equation. The fundamental properties of such nonlinear waves have been theoretically analyzed by comparing system potential for both positive and negative dust grains. It has been shown that the basic features of these waves are significantly modified by the positive and negative ions drift speed and polarities of dust grains. The implications of our results in space and laboratory plasmas are briefly discussed.
基金support from the National Natural Science Foundation of China(22090031,22090030,22288102),Qinghai Salt Lake Industry Group Co.,Ltd.
文摘Aqueous rechargeable batteries using abundant multi-ion cations have receivedincreasing attention in the energy storage field for their high safety and low cost.Layered double hydroxides(LDHs)possess a two-dimensional structure andexhibit great potential as cathodes for multi-ion intercalation.However,theinsufficient active sites of LDHs result in low capacities in the discharging process.Interestingly,the LDHs after the deprotonation process exhibit favorable electrochemicalperformance of multi-cation intercalation.The deprotonation process ofLDHs has been widely found in the oxygen evolution reaction and energy storagefield,where LDHs lose H in laminates and converts to deprotonatedγ-phaseMOOHs(MOOs).Herein,we take a comprehensive overview of the dynamicsstructure transformation of the deprotonation process of LDHs.Furthermore,thedevelopment of advanced aqueous battery cathode and metal battery anode basedon deprotonated LDHs for energy storage is explored and summarized.Finally,theperspective of deprotonated LDHs in the energy storage field is discussed.
基金The authors would like to acknowledge financial support from the National Key R&D Program of China(Nos.2021YFF1200700 and 2021YFA0911100)the National Natural Science Foundation of China(Nos.T2225010,32171399,and 32171456)+4 种基金the Fundamental Research Funds for the Central Universities,Sun Yat-Sen University(No.22dfx02)Pazhou Lab,Guangzhou(No.PZL2021KF0003)The authors also would like to thank the funding support from the Opening Project of Key Laboratory of Microelectronic Devices&Integrated Technology,Institute of Microelectronics,Chinese Academy of Sciences,and State Key Laboratory of Precision Measuring Technology and Instruments(No.pilab2211)QQOY would like to thank the China Postdoctoral Science Foundation(No.2022M713645)JL would like to thank the National Natural Science Foundation of China(No.62105380)and the China Postdoctoral Science Foundation(No.2021M693686).
文摘Modern medicine is increasingly interested in advanced sensors to detect and analyze biochemical indicators.Ion sensors based on potentiometric methods are a promising platform for monitoring physiological ions in biological subjects.Current semi-implantable devices are mainly based on single-parameter detection.Miniaturized semi-implantable electrodes for multiparameter sensing have more restrictions on the electrode size due to biocompatibility considerations,but reducing the electrode surface area could potentially limit electrode sensitivity.This study developed a semi-implantable device system comprising a multiplexed microfilament electrode cluster(MMEC)and a printed circuit board for real-time monitoring of intra-tissue K^(+),Ca^(2+),and Na^(+)concentrations.The electrode surface area was less important for the potentiometric sensing mechanism,suggesting the feasibility of using a tiny fiber-like electrode for potentiometric sensing.The MMEC device exhibited a broad linear response(K^(+):2–32 mmol/L;Ca^(2+):0.5–4 mmol/L;Na^(+):10–160 mmol/L),high sensitivity(about 20–45 mV/decade),temporal stability(>2weeks),and good selectivity(>80%)for the above ions.In vitro detection and in vivo subcutaneous and brain experiment results showed that the MMEC system exhibits good multi-ion monitoring performance in several complex environments.This work provides a platform for the continuous real-time monitoring of ion fluctuations in different situations and has implications for developing smart sensors to monitor human health.
文摘面向电动汽车一类宽温度,大幅值、宽频率随机电流应用场景,提出一种基于全新电热耦合模型的锂电池多状态在线联合估计方法。该模型由自回归等效电路模型与单态集总热模型耦合而成,以提高模型电气动态跟随性能。电热耦合模型参数采取“先验信息初始化-在线修正”的方式确定,以避免电池一致性问题带来的误差,从而实现电热耦合关系在宽温度内的连续准确表达。基于所提出的ARST(autoregression-single state thermal model)耦合模型,该文采用双滤波算法实现锂电池多状态的在线联合估计,弥补目前电池3种及以上状态联合估计的稀缺问题。最后,在[0,50]℃,基于两个动态工况,将所提出的算法与两类基于模型的多状态联合估计算法进行比较。结果表明:ARST模型具有更好的电气跟随性能;所提出的模型参数在线辨识算法能够有效提高模型精度,从而提高多状态联合估计精度;在宽温度应用中,相较仅基于电模型的多状态联合估计算法,兼顾热状态估计的多状态联合估计算法能够有效提高电池状态的估计精度。
