Removing large concentrations of organic pollutants from water efficiently and quickly under visible light is essential to developing photocatalytic technology and improving solar energy efficiency.This study used a s...Removing large concentrations of organic pollutants from water efficiently and quickly under visible light is essential to developing photocatalytic technology and improving solar energy efficiency.This study used a simple hydrothermal method to prepare a non-metallic,S-doped NaTaO_(3)(S-NTO) photocatalyst,which was then loaded onto biochar (BC) to form a S-NTO/BC composite photocatalyst.After uniform loading onto BC,the S-NTO particles transformed from cubic to spherical.The photogenerated electron-hole pair recombination probability of the composite photocatalyst was significantly lower than those of the NTO particles.The light absorption range of the catalyst was effectively widened from 310 nm UV region to visible region.In addition,a dual-effect catalytic system was constructed by introducing peroxymonosulfate (PMS) into the environment of the pollution to be degraded.The Rhodamine B,Methyl Orange,Acid Orange 7,tetracycline,and ciprofloxacin degradation efficiency at 40 mg/L reached 99.6%,99.2%,84.5%,67.1%,and 70.7%,respectively,after irradiation by a 40 W lamps for 90 min.The high-efficiency visible-light catalytic activity of the dual-effect catalytic system was attributed to doping with non-metallic sulfur and loading of catalysts onto BC.The development of this dual-effect catalytic system provides new ideas for quickly and efficiently solving the problem of high-concentration organic pollution in aqueous environments,rationally and fully utilizing solar energy,and expanding the application of photocatalytic technology to practice.展开更多
该文提出黏滞阻尼与滞变阻尼共同作用的双阻尼模型调谐质量阻尼器(Dual Damping Tuned Mass Damper,DD-TMD),并对白噪声作用下DD-TMD进行减震优化研究。讨论了DD-TMD的构成、优势和应用范围,并总结了DD-TMD的力学机理。提出适用于DD-TMD...该文提出黏滞阻尼与滞变阻尼共同作用的双阻尼模型调谐质量阻尼器(Dual Damping Tuned Mass Damper,DD-TMD),并对白噪声作用下DD-TMD进行减震优化研究。讨论了DD-TMD的构成、优势和应用范围,并总结了DD-TMD的力学机理。提出适用于DD-TMD的H_(2)优化方法,并通过数值寻优得到了最优参数和基于稳定区域的DD-TMD参数优化方法。此外,通过DD-TMD的H_(2)优化方法进一步得到了DD-TMD的等效附加黏滞阻尼比,为工程设计奠定应用基础。以变摩擦摆式调谐质量阻尼器(Variable Friction Pendulum Tuned Mass Damper,VFP-TMD)为DD-TMD的实际应用算例,通过20条地震波检验所提出的优化方法对地震激励的减震性能影响。结果表明:H_(2)优化下的DD-TMD可以提供与常规黏滞阻尼TMD相当的控制效果。采用DD-TMD可以通过随机理论成功模拟与常摩擦阻尼等效的黏滞阻尼,并为带有初始摩擦的VFP-TMD提供有效可靠的优化设计方法。相较于前人所做的数值寻优方法,按照DD-TMD模型优化的VFP-TMD可以提供更加优异的减震控制效果且阻尼耗能能力提高了16.6%。展开更多
基金financially supported by the Science and Technology Major Project on Lakes of Inner Mongolia (No.ZDZX2018054)the National Natural Science Foundation of China for Less Developed Regions (No.51868054)+1 种基金Innovation Guide Project of Inner Mongolia Autonomous Region (No.KCBJ2018005)Inner Mongolia University special funds for postgraduate innovation and entrepreneurship (No.11200-121024)。
文摘Removing large concentrations of organic pollutants from water efficiently and quickly under visible light is essential to developing photocatalytic technology and improving solar energy efficiency.This study used a simple hydrothermal method to prepare a non-metallic,S-doped NaTaO_(3)(S-NTO) photocatalyst,which was then loaded onto biochar (BC) to form a S-NTO/BC composite photocatalyst.After uniform loading onto BC,the S-NTO particles transformed from cubic to spherical.The photogenerated electron-hole pair recombination probability of the composite photocatalyst was significantly lower than those of the NTO particles.The light absorption range of the catalyst was effectively widened from 310 nm UV region to visible region.In addition,a dual-effect catalytic system was constructed by introducing peroxymonosulfate (PMS) into the environment of the pollution to be degraded.The Rhodamine B,Methyl Orange,Acid Orange 7,tetracycline,and ciprofloxacin degradation efficiency at 40 mg/L reached 99.6%,99.2%,84.5%,67.1%,and 70.7%,respectively,after irradiation by a 40 W lamps for 90 min.The high-efficiency visible-light catalytic activity of the dual-effect catalytic system was attributed to doping with non-metallic sulfur and loading of catalysts onto BC.The development of this dual-effect catalytic system provides new ideas for quickly and efficiently solving the problem of high-concentration organic pollution in aqueous environments,rationally and fully utilizing solar energy,and expanding the application of photocatalytic technology to practice.
文摘该文提出黏滞阻尼与滞变阻尼共同作用的双阻尼模型调谐质量阻尼器(Dual Damping Tuned Mass Damper,DD-TMD),并对白噪声作用下DD-TMD进行减震优化研究。讨论了DD-TMD的构成、优势和应用范围,并总结了DD-TMD的力学机理。提出适用于DD-TMD的H_(2)优化方法,并通过数值寻优得到了最优参数和基于稳定区域的DD-TMD参数优化方法。此外,通过DD-TMD的H_(2)优化方法进一步得到了DD-TMD的等效附加黏滞阻尼比,为工程设计奠定应用基础。以变摩擦摆式调谐质量阻尼器(Variable Friction Pendulum Tuned Mass Damper,VFP-TMD)为DD-TMD的实际应用算例,通过20条地震波检验所提出的优化方法对地震激励的减震性能影响。结果表明:H_(2)优化下的DD-TMD可以提供与常规黏滞阻尼TMD相当的控制效果。采用DD-TMD可以通过随机理论成功模拟与常摩擦阻尼等效的黏滞阻尼,并为带有初始摩擦的VFP-TMD提供有效可靠的优化设计方法。相较于前人所做的数值寻优方法,按照DD-TMD模型优化的VFP-TMD可以提供更加优异的减震控制效果且阻尼耗能能力提高了16.6%。
