Tumor-targeted magnetic hyperthermia has recently attracted much attention.Magnetic nanoparticles(NPs) are heat mediator nanoprobes in magnetic hyperthermia for cancer treatment.In this paper,single cubic spinel struc...Tumor-targeted magnetic hyperthermia has recently attracted much attention.Magnetic nanoparticles(NPs) are heat mediator nanoprobes in magnetic hyperthermia for cancer treatment.In this paper,single cubic spinel structural Zn_(0.3)Fe_(2.7)O_(4) magnetic NPs with sizes of 14 nm-20 nm were synthesized,followed by coating with SiO_(2) shell.The SLP value of Zn_(0.3)Fe_(2.7)O_(4)/SiO_(2) NPs below 20 nm changes non-monotonically with the concentration of solution under the alternating current(AC) magnetic field of 430 kHz and 27 kA/m.SLP values of all Zn_(0.3)Fe_(2.7)O_(4)/SiO_(2) NPs appear a peak value with change of solution concentration.The solution concentrations with optimal SLP value decrease with increasing magnetic core size.This work can give guidance to the better prediction and control of the magnetic hyperthermia performance of materials in clinical applications.展开更多
We report on a forest-like-to-desert-like pattern evolution in the growth of an organic thin film observed by using an atomic force microscope. We use a modified diffusion limited aggregation model to simulate the gro...We report on a forest-like-to-desert-like pattern evolution in the growth of an organic thin film observed by using an atomic force microscope. We use a modified diffusion limited aggregation model to simulate the growth process and are able to reproduce the experimental patterns. The energy of electric dipole interaction is calculated and determined to be the driving force for the pattern formation and evolution. Based on these results, single crystalline films are obtained by enhancing the electric dipole interaction while limiting effects of other growth parameters.展开更多
Sound velocity, density, and viscosity values were measured at 303 K in four binary systems of benzene +1-, 2-, tert-, or iso-butanol. From these data, acoustical parameters, such as adiabatic compressibility, free le...Sound velocity, density, and viscosity values were measured at 303 K in four binary systems of benzene +1-, 2-, tert-, or iso-butanol. From these data, acoustical parameters, such as adiabatic compressibility, free length, free volume, and internal pressure were estimated using the standard relations. The results are interpreted in terms of molecular interaction between the components of the mixtures. Observed excess value in all the mixture indicates that the molecular symmetry existing in the system is highly disturbed by the nonpolar benzene molecules. Interaction energy terms of the statistical mixing are also verified for these binary systems and the dipole-dipole interactions are found to be predominantly present and are sharply affected by the isomeric forms of butanol.展开更多
SmCo/FeCo/SmCo trilayer was deposited with two different thickness configurations for soft phase (FeCo);50 nm/10 nm/50 nm and 50 nm/25 nm/50 nm were deposited on Si (111) substrate and Ta (50 nm) seed layer by RF magn...SmCo/FeCo/SmCo trilayer was deposited with two different thickness configurations for soft phase (FeCo);50 nm/10 nm/50 nm and 50 nm/25 nm/50 nm were deposited on Si (111) substrate and Ta (50 nm) seed layer by RF magnetron sputtering in a pressure, p, of 30 - 35 m Torr. After deposition the films were annealed under Ar atmosphere at temperature T equal to 923 and 973 for different times followed by quenching in water. X-ray diffraction patterns were obtained to identified phase presents and calculate average crystallite size. To study the effect of configuration thickness in soft phases, DC magnetic measurements were carried out;the measurements were done in the temperature interval of 300 - 50 K. Hysteresis loops collected at low temperatures exposed an increment in coercivity with the decrease of T and at same time, presented a “knee” in the second quadrant of the demagnetization curve, which suggests that the inter-layer exchange coupling becomes less effective, being more evident for sample with 50 nm/25 nm/50 nm thickness. Moreover, δM (H) plots were calculated from magnetic measurements at three different temperatures, T, equal to 300, 150 and 50 K, which corroborates that the dipolar interactions became stronger when thickness of soft phases increases. Finally, the thickness effect is attributed to the SmCo5 phase magnetocrystalline anisotropy constant, which is responsible for the exchange coupling length.展开更多
We study the formation of vortices in a dipolar Bose-Einstein condensate in a synthetic magnetic field by numerically solving the Gross-Pitaevskii equation. The formation process depends on the dipole strength, the ro...We study the formation of vortices in a dipolar Bose-Einstein condensate in a synthetic magnetic field by numerically solving the Gross-Pitaevskii equation. The formation process depends on the dipole strength, the rotating frequency, the potential geometry, and the orientation of the dipoles. We make an extensive comparison with vortices created by a rotating trap, especially focusing on the issues of the critical rotating frequency and the vortex number as a function of the rotating frequency. We observe that a higher rotating frequency is needed to generate a large number of vortices and the anisotropic interaction manifests itself as a perceptible difference in the vortex formation. Furthermore, a large dipole strength or aspect ratio also can increase the number of vortices effectively. In particular, we discuss the validity of the Feynman rule.展开更多
The determination of natural products stereochemistry remains a formidable task.Residual dipolar couplings(RDCs)induced by anisotropic media are a powerful tool for determination of the stereochemistry of organic mole...The determination of natural products stereochemistry remains a formidable task.Residual dipolar couplings(RDCs)induced by anisotropic media are a powerful tool for determination of the stereochemistry of organic molecule in solution.This review will provide a short introduction on RDCs-based methodology for the structural elucidation of natural products.Special attention is given to the current availability of alignment media in organic solvents.The applications of RDCs for structural analysis of some examples of natural products were discussed and summarized.Graphical Abstract This review provides a short introduction on RDCs-based methodology for the structural elucidation of natural products.Special attention is given to the current availability of alignment media in organic solvents.The applications of RDCs for structural analysis of some examples of natural products were discussed and summarized.展开更多
With conjunction observations of electromagnetic fields and plasma from Time History of Events and Macroscale Interactions during Substorm(THEMIS)in the near-Earth magnetotail,we investigate the spatial and temporal p...With conjunction observations of electromagnetic fields and plasma from Time History of Events and Macroscale Interactions during Substorm(THEMIS)in the near-Earth magnetotail,we investigate the spatial and temporal properties of substorm dipolarizations in the near-Earth plasma sheet(NEPS)during a substorm at 03:23 UT on 12 February 2008.Substorm dipolarizations with different features are detected by three near-Earth THEMIS probes(THA(P5),THD(P3)and THE(P4))in the magnetotail.In the current sheet with a large plasma beta value(β>2,whereβis the ratio of the plasma thermal pressure to the magnetic pressure),the dipolarization within the substorm onset region,(−10.4,2.8,−2.6)RE_gsm,has a large initial magnetic field elevation angle,θ>60°,θ=arctan(Bz/(Bx2+By2)1/2),and is accompanied by energetic ion(tens to hundred keV)dispersionless injection detected by THD(P3).This substorm onset dipolarization is characterized by Bx and By components around 0 nT with significant fluctuations.The Bz component increases sharply and its subsequent magnitude approaches the total magnetic field,Bt.The maximum value of the elevation angle approaches 85°during the later substorm expansion phase.In the NEPS withβ~1,the dipolarization outside the substorm onset region is characterized by a magnetic elevation angle with a small beginning value ofθ<45°and following multi-step enhancements during the substorm expansion phase.The maximum value of the elevation angle approaches to 70°during the later substorm expansion phase.Our observation results indicate that characteristics of dipolarization with a large beginning elevation angle within the substorm onset region provide a new indicator to identify substorm onset location.展开更多
A modified correlated spectroscopy （COSY） revamped with asymmetric Z-gradient echo detection sequence was designed to investigate the influence of diffusion hehaviour on intermolecular double-quantum coherence signa...A modified correlated spectroscopy （COSY） revamped with asymmetric Z-gradient echo detection sequence was designed to investigate the influence of diffusion hehaviour on intermolecular double-quantum coherence signal attenuation during the pre-acquisition period. Theoretical formulas were deduced and experimental measurements and simulations were performed. It is found that the diffusion behaviour of intermolecular double-quantum coherence in the pre-acquisition period may be different from that of conventional single-quantum coherence, depending on the relative orientation of diffusion weighting gradients to coherence selection gradients. When the orientation of the diffusion weighting gradients is parallel or anti-parallel to the orientation of the coherence selection gradients, the diffusion is modulated by the distant dipolar field. This study is helpful for understanding the signal properties in intermolecular double-quantum coherence magnetic resonance imaging.展开更多
Previous studies suggest that dipolarization fronts (DFs) are 1 to 3RE (RE is the earth radius) wide in the dawn-dusk direction. Recent kinetic simulations have found that DFs may break up into small-scale structures ...Previous studies suggest that dipolarization fronts (DFs) are 1 to 3RE (RE is the earth radius) wide in the dawn-dusk direction. Recent kinetic simulations have found that DFs may break up into small-scale structures after they are produced by reconnection. Motivated by this simulation, we revisited the scale size of DFs in the dawn-dusk direction by using Cluster observations during the years when the inter-distance among Cluster spacecraft was between 1000 and 2000 km. We selected the DFs that were detected by more than one spacecraft and estimated the radii of these DFs by a simple geometrical analysis, which is based on comparison of DF normals observed by different spacecraft. We found a few DFs that were only a few ion inertial lengths in the dawn-dusk direction. These results point out the importance of multi-scale coupling during the evolution of DFs.展开更多
1,4-Addition reaction of Grignard's reagent to 5-methoxy-2(5H)-furanone 1 was accomplished. which provided a new possible route for synthesizing beta -alkyl-Y-alkyloxy-Y-butyrolactone. A novel concise method of pr...1,4-Addition reaction of Grignard's reagent to 5-methoxy-2(5H)-furanone 1 was accomplished. which provided a new possible route for synthesizing beta -alkyl-Y-alkyloxy-Y-butyrolactone. A novel concise method of preparing fused heterocyclic compounds was offered by 1,3-dipolar cycloaddition reaction of silyl nitronates to 1.展开更多
facile one-step method is presented for the synthesis of indolizines in moder-ate to high yields by reaction of pyridinium, quinolinium and isoquinolinium ylideswith acrylonitrile, methyl acrylate and diethyl maleate ...facile one-step method is presented for the synthesis of indolizines in moder-ate to high yields by reaction of pyridinium, quinolinium and isoquinolinium ylideswith acrylonitrile, methyl acrylate and diethyl maleate respectively in the presenceof tetrakis-pyridino-cobalt(Ⅱ)dichromate (TPCD) in DMF.展开更多
We study quantum tunneling of a dipolar Bose-Einstein condensate in optical lattice when the spin system initially is prepared in a squeezed coherent state. It is found that there exists quantum tunneling between latt...We study quantum tunneling of a dipolar Bose-Einstein condensate in optical lattice when the spin system initially is prepared in a squeezed coherent state. It is found that there exists quantum tunneling between lattices l and l ＋ 1, l and l - 1, respectively. In particular, when the optical lattice is infinitely long and the spin excitations are in the long-wavelength limit, quantum tunneling disappears between lattices l and l ＋ 1, and that l and l - 1. Correspondingly, the magnetic soliton appears.展开更多
1 Introduction Fullerene has received considerable attention and a great researching interest due to its unique structure and interesting properties[1―3]. Many functional groups have been introduced, often region- or...1 Introduction Fullerene has received considerable attention and a great researching interest due to its unique structure and interesting properties[1―3]. Many functional groups have been introduced, often region- or stereo-selectively, for tuning the physical properties of C60and for constructing supramoleculararchitectures^[4-6].展开更多
We consider a binary dipolar Bose–Einstein condensate confined in a rotating harmonic plus quartic potential trap.The ground-state vortex structures are numerically obtained as a function of the contact interactions ...We consider a binary dipolar Bose–Einstein condensate confined in a rotating harmonic plus quartic potential trap.The ground-state vortex structures are numerically obtained as a function of the contact interactions and the dipole–dipole interaction in both slow and rapid rotation cases. The results show that the vortex configurations depend strongly on the strength of the contact interactions, the relative strength between dipolar and contact interactions, as well as on the orientation of the dipoles. A variety of exotic ground-state vortex structures, such as pentagonal and hexagon vortex lattice,square vortex lattice with a central vortex, annular vortex lines, and straight vortex lines, are observed by turning such controllable parameters. Our results deepen the understanding of effects of dipole–dipole interaction on the topological defects.展开更多
Reflection and transmission of an incident plane wave at five types of possible interfaces between two dipolar gradient elastic solids are studied in this paper. First, the explicit expressions of monopolar tractions ...Reflection and transmission of an incident plane wave at five types of possible interfaces between two dipolar gradient elastic solids are studied in this paper. First, the explicit expressions of monopolar tractions and dipolar tractions are derived from the postulated function of strain energy density. Then, the displacements, the normal derivative of displacements, monopolar tractions, and dipolar tractions are used to create the nontraditional interface conditions. There are five types of possible interfaces based on all possible combinations of the displacements and the normal derivative of displacements. These interfacial conditions with consideration of microstructure effects are used to determine the amplitude ratio of the reflection and transmission waves with respect to the incident wave. Further, the energy ratios of the reflection and transmission waves with respect to the incident wave are calculated. Some numerical results of the reflection and transmission coefficients are given in terms of energy flux ratio for five types of possible interfaces. The influences of the five types of possible interfaces on the energy partition between the refection waves and the transmission waves are discussed, and the concept of double channels of energy transfer is first proposed to explain the different influences of five types of interfaces.展开更多
Exact solutions for three canonical flow problems of a dipolar fluid are obtained: (i) The flow of a dipolar fluid due to a suddenly accelerated plate, (ii) The flow generated by periodic oscillation of a plate, (iii)...Exact solutions for three canonical flow problems of a dipolar fluid are obtained: (i) The flow of a dipolar fluid due to a suddenly accelerated plate, (ii) The flow generated by periodic oscillation of a plate, (iii) The flow due to plate oscillation in the presence of a transverse magnetic field. The solutions of some interesting flows caused by an arbitrary velocity of the plate and of certain special oscillations are also obtained.展开更多
Several isoxazoline compounds were obtained by the 1,3-dipolar cycloaddition of benzonitrile oxide to 5-(R)-(l-menthyloxy)-2(5H)-furanone. The reaction condition was investigated preliminarily, the structures of thes...Several isoxazoline compounds were obtained by the 1,3-dipolar cycloaddition of benzonitrile oxide to 5-(R)-(l-menthyloxy)-2(5H)-furanone. The reaction condition was investigated preliminarily, the structures of these compounds have been established via the analysis of NMR data(involved NOEID or HMBC) and the reaction seems occurred regioselectively.展开更多
We investigate the particle-hole pair excitations of dipolar molecules in an optical lattice, which can be described with an extended Bose-Hubbard model. For strong enough dipole-dipole interaction, the particle-hole ...We investigate the particle-hole pair excitations of dipolar molecules in an optical lattice, which can be described with an extended Bose-Hubbard model. For strong enough dipole-dipole interaction, the particle-hole pair excitations can form bound states in one and two dimensions. With decreasing dipole-dipole interaction, the energies of the bound states increase and merge into the particle-hole continuous spectrum gradually. The existence regions, the energy spectra and the wave functions of the bound states are carefully studied and the symmetries of the bound states are analyzed with group theory. For a given dipole-dipole interaction, the number of bound states varies in momentum space and a number distribution of the bound states is illustrated. We also discuss how to observe these bound states in future experiments.展开更多
When a Bose-Einstein condensate is set to rotate, superfluid vortices will be formed, which finally condense into a vortex lattice as the rotation frequency further increases. We show that the dipole-dipole interactio...When a Bose-Einstein condensate is set to rotate, superfluid vortices will be formed, which finally condense into a vortex lattice as the rotation frequency further increases. We show that the dipole-dipole interactions renormalize the short-range interaction strength and result in a distinction between interactions of parallel-polarized atoms and interactions of antiparallel-polarized atoms. This effect may lead to a spontaneous breakdown of the rapidly rotating Bose condensate into a novel anti-ferromagnetic-like vortex lattice. The upward-polarized Bose condensate forms a vortex lattice, which is staggered against a downward-polarized vortex lattice. A phase diagram related to the coupling strength is obtained.展开更多
We numerically study the interaction dynamics of two bright solitons with zero initial velocities in the one-dimensional dipolar Bose-Einstein condensates.Under different dipolar strengths,the two bright solitons can ...We numerically study the interaction dynamics of two bright solitons with zero initial velocities in the one-dimensional dipolar Bose-Einstein condensates.Under different dipolar strengths,the two bright solitons can merge into a breathing wave,and then split or propagate constantly after several oscillating periods.We quantitatively study the breathing frequency of wave after merging and the asymmetry property of solitons after splitting,and analyze their formation mechanism by the system's energy evolution.Also,the change of initial phase difference brings distinct effects on the soliton interaction.Our results provide insight into the new dynamical phenomena in dipolar systems and enrich the understanding for interaction between dipolar solitons.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant Nos.51771124,51571146,and 51701130)。
文摘Tumor-targeted magnetic hyperthermia has recently attracted much attention.Magnetic nanoparticles(NPs) are heat mediator nanoprobes in magnetic hyperthermia for cancer treatment.In this paper,single cubic spinel structural Zn_(0.3)Fe_(2.7)O_(4) magnetic NPs with sizes of 14 nm-20 nm were synthesized,followed by coating with SiO_(2) shell.The SLP value of Zn_(0.3)Fe_(2.7)O_(4)/SiO_(2) NPs below 20 nm changes non-monotonically with the concentration of solution under the alternating current(AC) magnetic field of 430 kHz and 27 kA/m.SLP values of all Zn_(0.3)Fe_(2.7)O_(4)/SiO_(2) NPs appear a peak value with change of solution concentration.The solution concentrations with optimal SLP value decrease with increasing magnetic core size.This work can give guidance to the better prediction and control of the magnetic hyperthermia performance of materials in clinical applications.
基金Project supported by the National Natural Science Foundation of China (Grant No.10774176)the National Basic Research Program of China (Grant No.2006CB806202)
文摘We report on a forest-like-to-desert-like pattern evolution in the growth of an organic thin film observed by using an atomic force microscope. We use a modified diffusion limited aggregation model to simulate the growth process and are able to reproduce the experimental patterns. The energy of electric dipole interaction is calculated and determined to be the driving force for the pattern formation and evolution. Based on these results, single crystalline films are obtained by enhancing the electric dipole interaction while limiting effects of other growth parameters.
文摘Sound velocity, density, and viscosity values were measured at 303 K in four binary systems of benzene +1-, 2-, tert-, or iso-butanol. From these data, acoustical parameters, such as adiabatic compressibility, free length, free volume, and internal pressure were estimated using the standard relations. The results are interpreted in terms of molecular interaction between the components of the mixtures. Observed excess value in all the mixture indicates that the molecular symmetry existing in the system is highly disturbed by the nonpolar benzene molecules. Interaction energy terms of the statistical mixing are also verified for these binary systems and the dipole-dipole interactions are found to be predominantly present and are sharply affected by the isomeric forms of butanol.
文摘SmCo/FeCo/SmCo trilayer was deposited with two different thickness configurations for soft phase (FeCo);50 nm/10 nm/50 nm and 50 nm/25 nm/50 nm were deposited on Si (111) substrate and Ta (50 nm) seed layer by RF magnetron sputtering in a pressure, p, of 30 - 35 m Torr. After deposition the films were annealed under Ar atmosphere at temperature T equal to 923 and 973 for different times followed by quenching in water. X-ray diffraction patterns were obtained to identified phase presents and calculate average crystallite size. To study the effect of configuration thickness in soft phases, DC magnetic measurements were carried out;the measurements were done in the temperature interval of 300 - 50 K. Hysteresis loops collected at low temperatures exposed an increment in coercivity with the decrease of T and at same time, presented a “knee” in the second quadrant of the demagnetization curve, which suggests that the inter-layer exchange coupling becomes less effective, being more evident for sample with 50 nm/25 nm/50 nm thickness. Moreover, δM (H) plots were calculated from magnetic measurements at three different temperatures, T, equal to 300, 150 and 50 K, which corroborates that the dipolar interactions became stronger when thickness of soft phases increases. Finally, the thickness effect is attributed to the SmCo5 phase magnetocrystalline anisotropy constant, which is responsible for the exchange coupling length.
基金supported by the National Natural Science Foundation of China(Grant No.11274039)the National Basic Research Program of China(Grant No.2013CB922002)the Fundamental Research Funds for the Central Universities of China
文摘We study the formation of vortices in a dipolar Bose-Einstein condensate in a synthetic magnetic field by numerically solving the Gross-Pitaevskii equation. The formation process depends on the dipole strength, the rotating frequency, the potential geometry, and the orientation of the dipoles. We make an extensive comparison with vortices created by a rotating trap, especially focusing on the issues of the critical rotating frequency and the vortex number as a function of the rotating frequency. We observe that a higher rotating frequency is needed to generate a large number of vortices and the anisotropic interaction manifests itself as a perceptible difference in the vortex formation. Furthermore, a large dipole strength or aspect ratio also can increase the number of vortices effectively. In particular, we discuss the validity of the Feynman rule.
基金co-supported by National Natural Science Foundation of China(21572164,U1504207)the Sino-German Center for Research Promotion(GZ1289).
文摘The determination of natural products stereochemistry remains a formidable task.Residual dipolar couplings(RDCs)induced by anisotropic media are a powerful tool for determination of the stereochemistry of organic molecule in solution.This review will provide a short introduction on RDCs-based methodology for the structural elucidation of natural products.Special attention is given to the current availability of alignment media in organic solvents.The applications of RDCs for structural analysis of some examples of natural products were discussed and summarized.Graphical Abstract This review provides a short introduction on RDCs-based methodology for the structural elucidation of natural products.Special attention is given to the current availability of alignment media in organic solvents.The applications of RDCs for structural analysis of some examples of natural products were discussed and summarized.
基金supported by the National Natural Science Foundation of China(NSFC)under grants 41731070,41674167,41574161the Strategic Pioneer Program on Space Science,Chinese Academy of Sciences,grants XDA15052500,XDA15350201 and XDA15011401the Specialized Research Fund for State Key Laboratories of China.
文摘With conjunction observations of electromagnetic fields and plasma from Time History of Events and Macroscale Interactions during Substorm(THEMIS)in the near-Earth magnetotail,we investigate the spatial and temporal properties of substorm dipolarizations in the near-Earth plasma sheet(NEPS)during a substorm at 03:23 UT on 12 February 2008.Substorm dipolarizations with different features are detected by three near-Earth THEMIS probes(THA(P5),THD(P3)and THE(P4))in the magnetotail.In the current sheet with a large plasma beta value(β>2,whereβis the ratio of the plasma thermal pressure to the magnetic pressure),the dipolarization within the substorm onset region,(−10.4,2.8,−2.6)RE_gsm,has a large initial magnetic field elevation angle,θ>60°,θ=arctan(Bz/(Bx2+By2)1/2),and is accompanied by energetic ion(tens to hundred keV)dispersionless injection detected by THD(P3).This substorm onset dipolarization is characterized by Bx and By components around 0 nT with significant fluctuations.The Bz component increases sharply and its subsequent magnitude approaches the total magnetic field,Bt.The maximum value of the elevation angle approaches 85°during the later substorm expansion phase.In the NEPS withβ~1,the dipolarization outside the substorm onset region is characterized by a magnetic elevation angle with a small beginning value ofθ<45°and following multi-step enhancements during the substorm expansion phase.The maximum value of the elevation angle approaches to 70°during the later substorm expansion phase.Our observation results indicate that characteristics of dipolarization with a large beginning elevation angle within the substorm onset region provide a new indicator to identify substorm onset location.
基金Project supported by the National Natural Science Foundation of China (Grant No 10875101)the Natural Science Foundation of Fujian Province, China (Grant No 2008J0028)
文摘A modified correlated spectroscopy （COSY） revamped with asymmetric Z-gradient echo detection sequence was designed to investigate the influence of diffusion hehaviour on intermolecular double-quantum coherence signal attenuation during the pre-acquisition period. Theoretical formulas were deduced and experimental measurements and simulations were performed. It is found that the diffusion behaviour of intermolecular double-quantum coherence in the pre-acquisition period may be different from that of conventional single-quantum coherence, depending on the relative orientation of diffusion weighting gradients to coherence selection gradients. When the orientation of the diffusion weighting gradients is parallel or anti-parallel to the orientation of the coherence selection gradients, the diffusion is modulated by the distant dipolar field. This study is helpful for understanding the signal properties in intermolecular double-quantum coherence magnetic resonance imaging.
基金supported by the National Natural Science Foundation of China (NSFC) under grant 41774154 and 41504123the Science Foundation of Jiangxi Province under grant 20122BAB21 2002+1 种基金the Nanchang University graduate innovation special fund project under grant CX2017106the Key Industry Innovation Chain of Shaanxi under grant 2018JQ4032
文摘Previous studies suggest that dipolarization fronts (DFs) are 1 to 3RE (RE is the earth radius) wide in the dawn-dusk direction. Recent kinetic simulations have found that DFs may break up into small-scale structures after they are produced by reconnection. Motivated by this simulation, we revisited the scale size of DFs in the dawn-dusk direction by using Cluster observations during the years when the inter-distance among Cluster spacecraft was between 1000 and 2000 km. We selected the DFs that were detected by more than one spacecraft and estimated the radii of these DFs by a simple geometrical analysis, which is based on comparison of DF normals observed by different spacecraft. We found a few DFs that were only a few ion inertial lengths in the dawn-dusk direction. These results point out the importance of multi-scale coupling during the evolution of DFs.
基金This work was supported by the NNSFC (No.29672004).
文摘1,4-Addition reaction of Grignard's reagent to 5-methoxy-2(5H)-furanone 1 was accomplished. which provided a new possible route for synthesizing beta -alkyl-Y-alkyloxy-Y-butyrolactone. A novel concise method of preparing fused heterocyclic compounds was offered by 1,3-dipolar cycloaddition reaction of silyl nitronates to 1.
文摘facile one-step method is presented for the synthesis of indolizines in moder-ate to high yields by reaction of pyridinium, quinolinium and isoquinolinium ylideswith acrylonitrile, methyl acrylate and diethyl maleate respectively in the presenceof tetrakis-pyridino-cobalt(Ⅱ)dichromate (TPCD) in DMF.
基金The project partly supported by National Natural Science Foundation of China under Grant No.10574060the Natural Science Foundation of Beijing under Grant No.1072010.
文摘We study quantum tunneling of a dipolar Bose-Einstein condensate in optical lattice when the spin system initially is prepared in a squeezed coherent state. It is found that there exists quantum tunneling between lattices l and l ＋ 1, l and l - 1, respectively. In particular, when the optical lattice is infinitely long and the spin excitations are in the long-wavelength limit, quantum tunneling disappears between lattices l and l ＋ 1, and that l and l - 1. Correspondingly, the magnetic soliton appears.
基金Supported by the National Natural Science Foundation of China(No.20402002)the Natural Science Foundation of Fujian Province,China (No.211J01031)+1 种基金the Project of Fujian Provincial Department of Education,China(No.JA11044)the Program for Excellent Young Researchers in Universities of Fujian Province,China(No.JA10056)
文摘1 Introduction Fullerene has received considerable attention and a great researching interest due to its unique structure and interesting properties[1―3]. Many functional groups have been introduced, often region- or stereo-selectively, for tuning the physical properties of C60and for constructing supramoleculararchitectures^[4-6].
基金Project supported by the Sichuan Province Education Department Key Natural Science Fund,China(Grant No.17ZA339)the Chongqing Research Program of Basic Research and Frontier Technology,China(Grant No.cstc2014jcyjA50016)the National Natural Science Foundation of China(Grant No.61504016)
文摘We consider a binary dipolar Bose–Einstein condensate confined in a rotating harmonic plus quartic potential trap.The ground-state vortex structures are numerically obtained as a function of the contact interactions and the dipole–dipole interaction in both slow and rapid rotation cases. The results show that the vortex configurations depend strongly on the strength of the contact interactions, the relative strength between dipolar and contact interactions, as well as on the orientation of the dipoles. A variety of exotic ground-state vortex structures, such as pentagonal and hexagon vortex lattice,square vortex lattice with a central vortex, annular vortex lines, and straight vortex lines, are observed by turning such controllable parameters. Our results deepen the understanding of effects of dipole–dipole interaction on the topological defects.
基金supported by the Fundamental Research Funds for the Central Universities (Grant FRF-BR-15-026A)the State science and technology support program (Grant 2013BAK12B08)+1 种基金the Hei Long Jiang Natural Science Fund (Grant B2015019)the National Natural Science Foundation of China (Grant 10972029)
文摘Reflection and transmission of an incident plane wave at five types of possible interfaces between two dipolar gradient elastic solids are studied in this paper. First, the explicit expressions of monopolar tractions and dipolar tractions are derived from the postulated function of strain energy density. Then, the displacements, the normal derivative of displacements, monopolar tractions, and dipolar tractions are used to create the nontraditional interface conditions. There are five types of possible interfaces based on all possible combinations of the displacements and the normal derivative of displacements. These interfacial conditions with consideration of microstructure effects are used to determine the amplitude ratio of the reflection and transmission waves with respect to the incident wave. Further, the energy ratios of the reflection and transmission waves with respect to the incident wave are calculated. Some numerical results of the reflection and transmission coefficients are given in terms of energy flux ratio for five types of possible interfaces. The influences of the five types of possible interfaces on the energy partition between the refection waves and the transmission waves are discussed, and the concept of double channels of energy transfer is first proposed to explain the different influences of five types of interfaces.
文摘Exact solutions for three canonical flow problems of a dipolar fluid are obtained: (i) The flow of a dipolar fluid due to a suddenly accelerated plate, (ii) The flow generated by periodic oscillation of a plate, (iii) The flow due to plate oscillation in the presence of a transverse magnetic field. The solutions of some interesting flows caused by an arbitrary velocity of the plate and of certain special oscillations are also obtained.
文摘Several isoxazoline compounds were obtained by the 1,3-dipolar cycloaddition of benzonitrile oxide to 5-(R)-(l-menthyloxy)-2(5H)-furanone. The reaction condition was investigated preliminarily, the structures of these compounds have been established via the analysis of NMR data(involved NOEID or HMBC) and the reaction seems occurred regioselectively.
基金supported by the National Basic Research Program of China (Grant Nos. 2011CB921502)the National Natural Science Foundation of China (Grant No. 10934010)+1 种基金the Joint Research Projects of the National Natural Science Foundation of ChinaHong Kong Research Grant Council (Grant Nos. 11061160490 and N-HKU748/10)
文摘We investigate the particle-hole pair excitations of dipolar molecules in an optical lattice, which can be described with an extended Bose-Hubbard model. For strong enough dipole-dipole interaction, the particle-hole pair excitations can form bound states in one and two dimensions. With decreasing dipole-dipole interaction, the energies of the bound states increase and merge into the particle-hole continuous spectrum gradually. The existence regions, the energy spectra and the wave functions of the bound states are carefully studied and the symmetries of the bound states are analyzed with group theory. For a given dipole-dipole interaction, the number of bound states varies in momentum space and a number distribution of the bound states is illustrated. We also discuss how to observe these bound states in future experiments.
基金The project supported by National Natural Science Foundation of China under Grant No. 10574012
文摘When a Bose-Einstein condensate is set to rotate, superfluid vortices will be formed, which finally condense into a vortex lattice as the rotation frequency further increases. We show that the dipole-dipole interactions renormalize the short-range interaction strength and result in a distinction between interactions of parallel-polarized atoms and interactions of antiparallel-polarized atoms. This effect may lead to a spontaneous breakdown of the rapidly rotating Bose condensate into a novel anti-ferromagnetic-like vortex lattice. The upward-polarized Bose condensate forms a vortex lattice, which is staggered against a downward-polarized vortex lattice. A phase diagram related to the coupling strength is obtained.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11875220 and 12047502)。
文摘We numerically study the interaction dynamics of two bright solitons with zero initial velocities in the one-dimensional dipolar Bose-Einstein condensates.Under different dipolar strengths,the two bright solitons can merge into a breathing wave,and then split or propagate constantly after several oscillating periods.We quantitatively study the breathing frequency of wave after merging and the asymmetry property of solitons after splitting,and analyze their formation mechanism by the system's energy evolution.Also,the change of initial phase difference brings distinct effects on the soliton interaction.Our results provide insight into the new dynamical phenomena in dipolar systems and enrich the understanding for interaction between dipolar solitons.
