To better understand the characteristics of air quality and the relationship between the chemical composition evolution and source variation,an intensive atmospheric campaign was conducted in Tianjin,a megacity of the...To better understand the characteristics of air quality and the relationship between the chemical composition evolution and source variation,an intensive atmospheric campaign was conducted in Tianjin,a megacity of the North China Plain,from 10 February to 6 March 2015.There were 20 days exceeding the threshold value of secondary Chinese Ambient Air Quality Standards for PM2.5(75 μg m-3,daily average over 24 h)during the study period.Five air pollution episodes were selected for investigation.During the pre-holiday pollution episode,NH^+_4,NO^-_3,and SO^(2-)_4 were more abundant,indicating that air pollution was caused by motor vehicle exhaust emissions and coal consumption under unfavorable meteorological conditions.During Chinese Lunar New Year's Eve,widespread use of fireworks resulted in extremely high aerosol concentrations.Firework displays caused increases in K+ and also enrichment of SO^(2-)_4 relative to NO^-_3.The holiday pollution episode was caused by regional transport,characterized by abundant SO^(2-)_4 and NH^+_4.In addition,the aging processes of the particles from fireworks discharge played an important role in the formation of NO-3and SO^(2-)_4.The Lantern Festival episode was characterized by a transition from the enrichment of K+ to secondary inorganic ions(NO^-_3,SO^(2-)_4,and NH^+_4).The results of this study are useful for a detailed understanding of the variation in atmospheric compositions and sources caused by anthropogenic activity,and highlight the importance of controlling intensive fireworks discharge.展开更多
The hallmark of development in the Yangtze River Delta(YRD) of East China has been sprawling urbanization. However, air pollution is a significant problem in these urban areas. In this paper, we investigated and analy...The hallmark of development in the Yangtze River Delta(YRD) of East China has been sprawling urbanization. However, air pollution is a significant problem in these urban areas. In this paper, we investigated and analyzed the air pollution index(API) in four cities(Shanghai, Nanjing, Hangzhou and Ningbo) in the YRD from 2001 to 2012. We attempted to empirically examine the relationship between meteorological factors and air quality in the urban areas of the YRD. According to the monitoring data, the API in Shanghai, Nanjing, Hangzhou slightly declined and that in Ningbo increased over the study period. We analyzed the inter-annual, seasonal, and monthly variations of API, from which we found that the air quality had different temporal changes in the four cities. It was indicated that air quality was poor in winter and spring and best in summer. Furthermore, different weather conditions affected air quality level. The wind direction was considered as an important and influential factor to air pollution, which has an impact on the accumulating or cleaning processes of pollutants. The air quality was influenced by the different wind directions that varied with seasons and cities.展开更多
基金supported by the Beijing Natural Science Foundation[grant number 8142034]Strategic Priority Research Program(B)of the Chinese Academy of Sciences[grant numbers XDB0502050 and XDB05030203]
文摘To better understand the characteristics of air quality and the relationship between the chemical composition evolution and source variation,an intensive atmospheric campaign was conducted in Tianjin,a megacity of the North China Plain,from 10 February to 6 March 2015.There were 20 days exceeding the threshold value of secondary Chinese Ambient Air Quality Standards for PM2.5(75 μg m-3,daily average over 24 h)during the study period.Five air pollution episodes were selected for investigation.During the pre-holiday pollution episode,NH^+_4,NO^-_3,and SO^(2-)_4 were more abundant,indicating that air pollution was caused by motor vehicle exhaust emissions and coal consumption under unfavorable meteorological conditions.During Chinese Lunar New Year's Eve,widespread use of fireworks resulted in extremely high aerosol concentrations.Firework displays caused increases in K+ and also enrichment of SO^(2-)_4 relative to NO^-_3.The holiday pollution episode was caused by regional transport,characterized by abundant SO^(2-)_4 and NH^+_4.In addition,the aging processes of the particles from fireworks discharge played an important role in the formation of NO-3and SO^(2-)_4.The Lantern Festival episode was characterized by a transition from the enrichment of K+ to secondary inorganic ions(NO^-_3,SO^(2-)_4,and NH^+_4).The results of this study are useful for a detailed understanding of the variation in atmospheric compositions and sources caused by anthropogenic activity,and highlight the importance of controlling intensive fireworks discharge.
基金Under the auspices of Special Research Fund of the Ministry of Land and Resources for the Non-Profit Sector(No201411014-03)National Key Technology Research and Development Program of China(No.2012BAH28B04)
文摘The hallmark of development in the Yangtze River Delta(YRD) of East China has been sprawling urbanization. However, air pollution is a significant problem in these urban areas. In this paper, we investigated and analyzed the air pollution index(API) in four cities(Shanghai, Nanjing, Hangzhou and Ningbo) in the YRD from 2001 to 2012. We attempted to empirically examine the relationship between meteorological factors and air quality in the urban areas of the YRD. According to the monitoring data, the API in Shanghai, Nanjing, Hangzhou slightly declined and that in Ningbo increased over the study period. We analyzed the inter-annual, seasonal, and monthly variations of API, from which we found that the air quality had different temporal changes in the four cities. It was indicated that air quality was poor in winter and spring and best in summer. Furthermore, different weather conditions affected air quality level. The wind direction was considered as an important and influential factor to air pollution, which has an impact on the accumulating or cleaning processes of pollutants. The air quality was influenced by the different wind directions that varied with seasons and cities.
