离子引出过程是原子蒸气激光同位素分离中非常重要的物理过程之一,而其中关键的等离子体参数(等离子体初始密度和电子温度等)均会对离子引出特性产生影响.基于千赫兹电源驱动的氩气高压交流放电等离子体射流源,建立了离子引出模拟实验平...离子引出过程是原子蒸气激光同位素分离中非常重要的物理过程之一,而其中关键的等离子体参数(等离子体初始密度和电子温度等)均会对离子引出特性产生影响.基于千赫兹电源驱动的氩气高压交流放电等离子体射流源,建立了离子引出模拟实验平台-2015 (IEX-2015),开发了用于诊断氩等离子体参数的"碰撞-辐射"模型,对等离子体射流区的电子温度和电子数密度等关键参数进行了测量.结果表明,电源输入功率和驱动频率以及工作气体流量均会对等离子体射流区的电子温度和数密度产生影响;在真空腔压强为10^(-2)Pa量级下,射流区电子数密度和电子温度的可调参数范围分别为10~9—10^(11)cm^(-3)和1.7—2.8 e V,这与实际离子引出过程中的等离子体参数范围相近.在此基础上,开展了不同引出电压、极板间距和电子数密度条件下初步的离子引出实验,所得到的离子引出电流变化规律亦与实际原子蒸气激光同位素分离中的离子引出特性定性一致.上述研究结果验证了在IEX-2015上开展离子引出模拟实验的可行性,为后续深入开展离子引出特性的实验研究准备了良好的条件.展开更多
In this work, experiment investigations and simulation studies of a waveguide-based microwave plasma source operated at 2.45 GHz in atmospheric pressure helium gas are presented. The plasma source has been designed in...In this work, experiment investigations and simulation studies of a waveguide-based microwave plasma source operated at 2.45 GHz in atmospheric pressure helium gas are presented. The plasma source has been designed in conjunction with a gas spectrograph as a speciation analysis tool. Emitted He spectra are observed for gas flow rates between (0.2-1) L/min and microwave power in the range (15-150) W. The results obtained demonstrate maximum excitation temperature of about 3800 K and gas temperature of about 2000 K. Mixtures containing small amounts of mercury atoms are considered and the resonant emission of Hg atoms at 253.56 nm is detected. The spectroscopic measurements are completed with a collisional radiative model delivering the electron density and temperature, the amplitude of the electric microwave field, and the population of the excited atomic states for a given absorbed power and gas temperature, The electromagnetic field distribution in the plasma source is obtained by solving Maxwell's equations. Electric field strength of several 10^5 V/m is obtained that agrees well with the results of the collisional radiative model. The calculated and measured line intensity ratios of He spectral lines agree within 300/0-40%.展开更多
文摘离子引出过程是原子蒸气激光同位素分离中非常重要的物理过程之一,而其中关键的等离子体参数(等离子体初始密度和电子温度等)均会对离子引出特性产生影响.基于千赫兹电源驱动的氩气高压交流放电等离子体射流源,建立了离子引出模拟实验平台-2015 (IEX-2015),开发了用于诊断氩等离子体参数的"碰撞-辐射"模型,对等离子体射流区的电子温度和电子数密度等关键参数进行了测量.结果表明,电源输入功率和驱动频率以及工作气体流量均会对等离子体射流区的电子温度和数密度产生影响;在真空腔压强为10^(-2)Pa量级下,射流区电子数密度和电子温度的可调参数范围分别为10~9—10^(11)cm^(-3)和1.7—2.8 e V,这与实际离子引出过程中的等离子体参数范围相近.在此基础上,开展了不同引出电压、极板间距和电子数密度条件下初步的离子引出实验,所得到的离子引出电流变化规律亦与实际原子蒸气激光同位素分离中的离子引出特性定性一致.上述研究结果验证了在IEX-2015上开展离子引出模拟实验的可行性,为后续深入开展离子引出特性的实验研究准备了良好的条件.
文摘In this work, experiment investigations and simulation studies of a waveguide-based microwave plasma source operated at 2.45 GHz in atmospheric pressure helium gas are presented. The plasma source has been designed in conjunction with a gas spectrograph as a speciation analysis tool. Emitted He spectra are observed for gas flow rates between (0.2-1) L/min and microwave power in the range (15-150) W. The results obtained demonstrate maximum excitation temperature of about 3800 K and gas temperature of about 2000 K. Mixtures containing small amounts of mercury atoms are considered and the resonant emission of Hg atoms at 253.56 nm is detected. The spectroscopic measurements are completed with a collisional radiative model delivering the electron density and temperature, the amplitude of the electric microwave field, and the population of the excited atomic states for a given absorbed power and gas temperature, The electromagnetic field distribution in the plasma source is obtained by solving Maxwell's equations. Electric field strength of several 10^5 V/m is obtained that agrees well with the results of the collisional radiative model. The calculated and measured line intensity ratios of He spectral lines agree within 300/0-40%.