We find that effects resulting from micro/nano scale structures can regulate space charges which excite and lead to the special electric field distribution featuring the flux convergence band structure. It is here ref...We find that effects resulting from micro/nano scale structures can regulate space charges which excite and lead to the special electric field distribution featuring the flux convergence band structure. It is here referred to as the polarization band effect, which stems from the specific field-induced interactions among atoms and molecules. The micro/nanoelectrode array structures were designed and fabricated using the non-silicon micro/nano processing technology, forming micro/nano electrode arrays-based plasma microelectromechanical systems(NPMEMS). The integrated NPMEMS device can be used to regulate the inner energy states of matters and generate plasma based on the polarization band effect, all within a single chip-size limited local area or extending into a large volume space with the deployment of a distributed array of multiple devices. Its special physical and chemical properties can be utilized to greatly improve the efficiency of potential application systems or solve mechanism-level challenges in plasma-related applications of multiple fields.展开更多
Propylene carbonate (PC) has a great potential to be used as an energy storage medium in the compact pulsed power sources due to its high dielectric constant and large resistivity. We investigate both the positive a...Propylene carbonate (PC) has a great potential to be used as an energy storage medium in the compact pulsed power sources due to its high dielectric constant and large resistivity. We investigate both the positive and negative breakdown characteristics of PC. The streamer patterns are obtained by ultra-high-speed cameras. The experimental results show that the positive breakdown voltage of PC is about 135% higher than the negative one, which is abnormal compared with the common liquid. The shape of the positive streamer is filamentary and branchy, while the negative streamer is tree-like and less branched. According to these experimental results, a charge layer structure model at the interface between the metal electrode and liquid is presented. It is suggested that the abnormal polarity effect basically arises from the electric field strength difference in the interface between both electrodes and PC. What is more, the recombination radiation and photoionization also play an important role in the whole discharge process.展开更多
Unconventional hydrocarbon reserves substantially surpass those of conventional resources and therefore are extremely economically attractive. However, exploration and production of uncon-ventional reserves is challen...Unconventional hydrocarbon reserves substantially surpass those of conventional resources and therefore are extremely economically attractive. However, exploration and production of uncon-ventional reserves is challenging. This paper demonstrates that one can observe significant induced polarization effects in shale reservoir rocks, which can be used in exploration for unconventional reserves. The generalized effective-medium theory of induced polarization (GEMTIP) was used to model the complex resistivity of shale rocks. We demonstrate that GEMTIP modeling provides an evaluation of mineral composition and volume fractions in rock samples. We have conducted spectral induced polarization (IP) measurements using different types of shale rocks to test the feasibility of the IP method and GEMTIP modeling for studying unconventional hydrocarbon (HC) reservoir rocks.展开更多
In order to study the polar substituent effect almost with no steric effect in organophosphorus chemistry,a series of 4-substituted-2,6,7-trioxa-1-phosphabicyclo[2.2.2]octane 1-oxides(1)and p-substituted phenylphospho...In order to study the polar substituent effect almost with no steric effect in organophosphorus chemistry,a series of 4-substituted-2,6,7-trioxa-1-phosphabicyclo[2.2.2]octane 1-oxides(1)and p-substituted phenylphosphonates(2)and corresponding mono hexyl esters(3)as model were synthesized.^(31)P-NMR chemical shifts of compounds(1)in methanol and deuterioacetone were determined.The Δδ values reflect 4-sbstituent po- lar effect.The ^(31)P-NMR of compounds(2)and(3)and the pKa of compounds(3)were also measured.The results showed that the trend of polar effects of substituents in both carboxylic and organophosphates chemistry are similar,and the change of polar effects in variation with the alkyl groups is not significant.展开更多
In this paper, we present a two-dimensional (2D) fully analytical model with consideration of polarization effect for the channel potential and electric field distributions of the gate field-plated high electron mob...In this paper, we present a two-dimensional (2D) fully analytical model with consideration of polarization effect for the channel potential and electric field distributions of the gate field-plated high electron mobility transistor (FP-HEMT) on the basis of 2D Poisson's solution. The dependences of the channel potential and electric field distributions on drain bias, polarization charge density, FP structure parameters, A1GaN/GaN material parameters, etc. are investigated. A simple and convenient approach to designing high breakdown voltage FP-HEMTs is also proposed. The validity of this model is demonstrated by comparison with the numerical simulations with Silvaco-Atlas. The method in this paper can be extended to the development of other analytical models for different device structures, such as MIS-HEMTs, multiple-FP HETMs, slant-FP HEMTs, etc.展开更多
The physical effects on surface and flexoelectric polarization in a weak anchoring nematic liquid crystal cell are investigated systematically. We derive the analytic expressions of two effective anchoring energies fo...The physical effects on surface and flexoelectric polarization in a weak anchoring nematic liquid crystal cell are investigated systematically. We derive the analytic expressions of two effective anchoring energies for lower and upper substrates respectively as well as their effective anchoring strengths and corresponding tilt angles of effective easy direction.All of these quantities are relevant to the magnitudes of both two polarizations and the applied voltage U. Based on these expressions, the variations of effective anchoring strength and the tilt angle with the applied voltage are calculated for the fixed values of two polarizations. For an original weak anchoring hybrid aligned nematic cell, it may be equivalent to a planar cell for a small value of U and has a threshold voltage. The variation of reduced threshold voltage with reduced surface polarization strength is also calculated. The role of surface polarization is important without the adsorptive ions considered.展开更多
We report on the temperature-dependent dc performance of A1GaN/GaN polarization doped field effect transistors (PolFETs). The rough decrements of drain current and transeonductance with the operation temperature are...We report on the temperature-dependent dc performance of A1GaN/GaN polarization doped field effect transistors (PolFETs). The rough decrements of drain current and transeonductance with the operation temperature are observed. Compared with the conventional HFETs, the drain current drop of the PolFET is smaller. The transeonductance drop of PolFETs at different gate biases shows different temperature dependences. From the aspect of the unique carrier behaviors of graded AlGaN/GaN heterostructure, we propose a quasi-multi-channel model to investigate the physics behind the temperature-dependent performance of AlGaN/GaN PolFETs.展开更多
In this paper we study the gain saturation induced mode-coupling control in solid state ring laser devices based on the stimulated Raman effect of the polar crystals in.order to realize solid state ring laser gyroscop...In this paper we study the gain saturation induced mode-coupling control in solid state ring laser devices based on the stimulated Raman effect of the polar crystals in.order to realize solid state ring laser gyroscopes. We theoretically investigate the mode coupling induced by gain saturation between clockwise (CW) and counterclockwise (CCW) propa- gating laser modes. Because the CW and CCW running waves are pumped with counter-propagating lasers respectively, the independent coexistence can be ensured.展开更多
Organic ferroelectric field-effect transistors (OFeFETs) are regarded as a promising technology for low-cost flexible memories. However, the electrical instability is still a critical obstacle, which limits the comm...Organic ferroelectric field-effect transistors (OFeFETs) are regarded as a promising technology for low-cost flexible memories. However, the electrical instability is still a critical obstacle, which limits the commercialization process. Based on already established models for polarization in ferroelectrics and charge transport in OFeFETs, simulation work is performed to determine the influence of polarization fatigue and ferroelectric switching transient on electrical characteristics in OFeFETs. The polarization fatigue results in the decrease of the on-state drain current and the memory window width and thus degrades the memory performance. The output measurements during the ferroelectric switching process show a hysteresis due to the instable polarization. In the on/off measurements, a large writing/erasing pulse frequency weakens the polarization modulation and thus results in a small separation between on- and off-state drain currents. According to the electrical properties of the ferroelectric layer, suggestions are given to obtain optimal electrical characterization for OFeFETs.展开更多
The effects of the protic and aprotic polar solvents on the emission spectrum of the naphthalene-triethyl-amine system in THF were studied under conditions of steady-state illumination. The fluorescence spectrum of th...The effects of the protic and aprotic polar solvents on the emission spectrum of the naphthalene-triethyl-amine system in THF were studied under conditions of steady-state illumination. The fluorescence spectrum of the naphthalene-triethylamine system consists of two emission bands, the fluorescence band of naphthalene(band A, 329 nm) and the emission band of the exciplex(band B, 468 nm). The intensities of both the emission bands decrease with increasing the solvent polarity. The intensity of band B also decreases due to the hydrogen-bonding interaction between triethylamine and protic solvent, while that of band A increases. It is thus suggested that the quenching of naphthalene fluorescence by triethylamine in THF occurs through the charge transfer and electron transfer reactions. The spectral changes upon the increase of solvent polarity can be explained by the dependences of the equilibrium constant between exciplex and ion-pair and the rate constant for the electron transfer reaction from triethylamine to the excited naphthalene on the relative permittivity of solvent. It is shown that the formation of intermolecular hydrogen-bonding between triethylamine and protic solvent suppresses the quenching reaction by the decrease in free amine. Acetonitrile has only a polar effect and trichloroacetic acid only a hydrogen-bonding(or protonation) effect, while alcohols have both the effects. The effects of alcohols could be separated into the effects of solvent polarity and intermolecular hydrogen-bonding interaction quantitatively.展开更多
To figure out the influence of isotope effect on product polarizations of the N(2D)+D2 reactive system and its isotope variants, quasi-classical trajectory(QCT) calculation was performed on Ho's potential energy...To figure out the influence of isotope effect on product polarizations of the N(2D)+D2 reactive system and its isotope variants, quasi-classical trajectory(QCT) calculation was performed on Ho's potential energy surface(PES) of 2A″ state. Product polarizations such as product distributions of P(θr), P(φr) and P(θr,φr), as well as the generalized polarization-dependent differential cross sections(PDDCSs) were discussed and compared in detail among the four product channels of the title reactions. Both the intermolecular and intramolecular isotope effects were proved to be influential on product polarizations.展开更多
Target micromotion not only plays an important role in target recognition but also leads to esoteric characteristics in synthetic aperture radar (SAR) imaging. This paper finds out an interesting phenomenon, i.e. th...Target micromotion not only plays an important role in target recognition but also leads to esoteric characteristics in synthetic aperture radar (SAR) imaging. This paper finds out an interesting phenomenon, i.e. the angular extent effect, in micro-motion target images formulated by the polar format algorithm. A micromotion target takes on multiple pairs of paired echoes (PEs) around the true point, and each PE extends for an angle which is exactly equal to the angular extent of the synthetic aperture, regardless of the micromotion frequency. The effect is derived and interpreted by using the characteristics of Bessel functions. Then it is demonstrated by simulation experiments of a target with different micromotion frequencies. The revelation and interpretation of the effect is highly beneficial to micromotion-target SAR image understanding as wel as target recognition.展开更多
We perform an experimental study of the multi-orbital effect on the high-order harmonic generation(HHG) from aligned N_2 molecules in both linearly and elliptically polarized intense laser fields.Measured by a home-bu...We perform an experimental study of the multi-orbital effect on the high-order harmonic generation(HHG) from aligned N_2 molecules in both linearly and elliptically polarized intense laser fields.Measured by a home-built extreme ultraviolet(XUV) flat grating spectrometer with the pump-probe method, the angular distributions of different orders of HHG are obtained, which show distinctive behaviors for harmonics in the plateau and the cut-off regions.The ellipticity dependence of HHG is investigated by aligning the molecular axis parallel or perpendicular to the laser polarization.Our results indicate that both the highest occupied molecular orbital(HOMO) as well as the lower one(HOMO-1) contribute to the HHG of N2 molecules, in either linearly or elliptically polarized intense laser field.The study paves the way for understanding the ultrafast electron dynamics of molecules exposed to an intense laser field.展开更多
A novel optimal design of sub-wavelength metal rectangular gratings for the polarizing beam splitter (PBS) is proposed. The method is based on effective medium theory and the method of designing single layer antiref...A novel optimal design of sub-wavelength metal rectangular gratings for the polarizing beam splitter (PBS) is proposed. The method is based on effective medium theory and the method of designing single layer antireflection coating. The polarization performance of PBS is discussed by rigorous couple-wave analysis (RCWA) method at a wavelength of 1550 nm. The result shows that sub-wavelength metal rectangular grating is characterized by a high reflectivity, like metal films for TE polarization, and high transmissivity, like dielectric films for TM polarization. The optimal design accords well with the results simulated by RCWA method.展开更多
The underlying mechanism of the spectral cleaning effect of the cross-polarized wave(XPW) generation process was theoretically investigated. This study shows that the spectral noise of an input spectrum can be remov...The underlying mechanism of the spectral cleaning effect of the cross-polarized wave(XPW) generation process was theoretically investigated. This study shows that the spectral noise of an input spectrum can be removed in the XPW generation process and that the spectral cleaning effect depends on the characteristics of the input pulses, such as the chirp and Fourier-transform-limited duration of the initial pulse, and the modulation amplitude and frequency of the spectral noise. Though these factors codetermine the output spectrum of the XPW generation process, the spectral cleaning effect is mainly affected by the initial pulse chirp. The smoothing of the spectrum in the XPW generation process leads to a significant enhancement of the coherent contrast.展开更多
We investigate atomic above-threshold ionization in elliptically polarized strong laser fields with a semiclassical approach.With increasing laser intensity,the Coulomb focusing(CF) effects are found to become stron...We investigate atomic above-threshold ionization in elliptically polarized strong laser fields with a semiclassical approach.With increasing laser intensity,the Coulomb focusing(CF) effects are found to become stronger in both parallel and perpendicular directions with respect to the polarization plane.The dependence of CF effects on tunnel exit,initial transverse momentum distribution and laser electric field is analyzed.It was revealed that the effects of tunnel exit are most prominent with variation of the laser intensity,and the other two factors both play non-negligible roles.Our results provide a deeper insight to the recent experiments of Coulomb asymmetry[Shafir D,et al.,2013 Phys.Rev.Lett.111 023005 and Li M,et al,2013 Phys.Rev.Lett.111 023006].展开更多
Analyzing powers and differential cross sections have been measured for elastic scattering of 22MeV polarized protons from 40Ca, 16O and 12C, and differential cross sections for inelastic scattering of 22 MeV protons ...Analyzing powers and differential cross sections have been measured for elastic scattering of 22MeV polarized protons from 40Ca, 16O and 12C, and differential cross sections for inelastic scattering of 22 MeV protons from 3- (3.736 MeV) and 5-(4.491 MeV) states of 40Ca have also been measured. The experimental data for polarized proton elastic scattering have been analyzed with a phenomenological optical potential parameters, the experimental data and theoretical values are in good agreement. In the theoretical frame of microscopic single scattering model, transition densities extracted from electron inelastic scattering and M3Y and Halderson’s effective interactions have been utilized to analyze the experimental data of 22 MeV proton inelastic scattering from 40Ca. Overall, it seems that Halderson’s effective interaction can better describe the experimental data than M3Y although the degree of agreement between experimental and theoretical values needs to he improved.展开更多
By making use of the quasi-two-dimensional (quasi-2D) model, the current-voltage (l-V) characteristics of In0AsA10.82N/A1N/GaN heterostructure field-effect transistors (HFETs) with different gate lengths are sim...By making use of the quasi-two-dimensional (quasi-2D) model, the current-voltage (l-V) characteristics of In0AsA10.82N/A1N/GaN heterostructure field-effect transistors (HFETs) with different gate lengths are simulated based on the measured capacitance-voltage (C-V) characteristics and I-V characteristics. By analyzing the variation of the electron mobility for the two-dimensional electron gas (2DEG) with electric field, it is found that the different polarization charge distributions generated by the different channel electric field distributions can result in different polarization Coulomb field scatterings. The difference between the electron mobilities primarily caused by the polarization Coulomb field scatterings can reach up to 1522.9 cm2/V.s for the prepared In0.38AI0.82N/A1N/GaN HFETs. In addition, when the 2DEG sheet density is modulated by the drain-source bias, the electron mobility presents a peak with the variation of the 2DEG sheet density, the gate length is smaller, and the 2DEG sheet density corresponding to the peak point is higher.展开更多
基金supported by the National Natural Science Foundationof China(60906053,61204069,61274118,61306144,61504079,and 11605112)Scientific and Innovative Action Plan of Shanghai(15DZ1160800 and 17XD1702400)National Key Research&Development(R&D)Program of China(Grant No.SQ2023YFC2600062).
文摘We find that effects resulting from micro/nano scale structures can regulate space charges which excite and lead to the special electric field distribution featuring the flux convergence band structure. It is here referred to as the polarization band effect, which stems from the specific field-induced interactions among atoms and molecules. The micro/nanoelectrode array structures were designed and fabricated using the non-silicon micro/nano processing technology, forming micro/nano electrode arrays-based plasma microelectromechanical systems(NPMEMS). The integrated NPMEMS device can be used to regulate the inner energy states of matters and generate plasma based on the polarization band effect, all within a single chip-size limited local area or extending into a large volume space with the deployment of a distributed array of multiple devices. Its special physical and chemical properties can be utilized to greatly improve the efficiency of potential application systems or solve mechanism-level challenges in plasma-related applications of multiple fields.
基金Supported by the National Natural Science Foundation of China under Grant No 51677190the Hunan Provincial Natural Science Foundation of China under Grant No 2017JJ1005
文摘Propylene carbonate (PC) has a great potential to be used as an energy storage medium in the compact pulsed power sources due to its high dielectric constant and large resistivity. We investigate both the positive and negative breakdown characteristics of PC. The streamer patterns are obtained by ultra-high-speed cameras. The experimental results show that the positive breakdown voltage of PC is about 135% higher than the negative one, which is abnormal compared with the common liquid. The shape of the positive streamer is filamentary and branchy, while the negative streamer is tree-like and less branched. According to these experimental results, a charge layer structure model at the interface between the metal electrode and liquid is presented. It is suggested that the abnormal polarity effect basically arises from the electric field strength difference in the interface between both electrodes and PC. What is more, the recombination radiation and photoionization also play an important role in the whole discharge process.
文摘Unconventional hydrocarbon reserves substantially surpass those of conventional resources and therefore are extremely economically attractive. However, exploration and production of uncon-ventional reserves is challenging. This paper demonstrates that one can observe significant induced polarization effects in shale reservoir rocks, which can be used in exploration for unconventional reserves. The generalized effective-medium theory of induced polarization (GEMTIP) was used to model the complex resistivity of shale rocks. We demonstrate that GEMTIP modeling provides an evaluation of mineral composition and volume fractions in rock samples. We have conducted spectral induced polarization (IP) measurements using different types of shale rocks to test the feasibility of the IP method and GEMTIP modeling for studying unconventional hydrocarbon (HC) reservoir rocks.
基金Project Supported by National Science Foundation of China.
文摘In order to study the polar substituent effect almost with no steric effect in organophosphorus chemistry,a series of 4-substituted-2,6,7-trioxa-1-phosphabicyclo[2.2.2]octane 1-oxides(1)and p-substituted phenylphosphonates(2)and corresponding mono hexyl esters(3)as model were synthesized.^(31)P-NMR chemical shifts of compounds(1)in methanol and deuterioacetone were determined.The Δδ values reflect 4-sbstituent po- lar effect.The ^(31)P-NMR of compounds(2)and(3)and the pKa of compounds(3)were also measured.The results showed that the trend of polar effects of substituents in both carboxylic and organophosphates chemistry are similar,and the change of polar effects in variation with the alkyl groups is not significant.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.61204085 and 61334002)the Fundamental Research Funds for the Central Universities,China(Grant No.K5051225013)
文摘In this paper, we present a two-dimensional (2D) fully analytical model with consideration of polarization effect for the channel potential and electric field distributions of the gate field-plated high electron mobility transistor (FP-HEMT) on the basis of 2D Poisson's solution. The dependences of the channel potential and electric field distributions on drain bias, polarization charge density, FP structure parameters, A1GaN/GaN material parameters, etc. are investigated. A simple and convenient approach to designing high breakdown voltage FP-HEMTs is also proposed. The validity of this model is demonstrated by comparison with the numerical simulations with Silvaco-Atlas. The method in this paper can be extended to the development of other analytical models for different device structures, such as MIS-HEMTs, multiple-FP HETMs, slant-FP HEMTs, etc.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11274088,11374087,and11304074)the Natural Science Foundation of Hebei Province,China(Grant No.A2014202123)+1 种基金the Research Project of Hebei Provincial Education Department,China(Grant No.QN2014130)the Key Subject Construction Project of Hebei Provincial University,China
文摘The physical effects on surface and flexoelectric polarization in a weak anchoring nematic liquid crystal cell are investigated systematically. We derive the analytic expressions of two effective anchoring energies for lower and upper substrates respectively as well as their effective anchoring strengths and corresponding tilt angles of effective easy direction.All of these quantities are relevant to the magnitudes of both two polarizations and the applied voltage U. Based on these expressions, the variations of effective anchoring strength and the tilt angle with the applied voltage are calculated for the fixed values of two polarizations. For an original weak anchoring hybrid aligned nematic cell, it may be equivalent to a planar cell for a small value of U and has a threshold voltage. The variation of reduced threshold voltage with reduced surface polarization strength is also calculated. The role of surface polarization is important without the adsorptive ions considered.
文摘We report on the temperature-dependent dc performance of A1GaN/GaN polarization doped field effect transistors (PolFETs). The rough decrements of drain current and transeonductance with the operation temperature are observed. Compared with the conventional HFETs, the drain current drop of the PolFET is smaller. The transeonductance drop of PolFETs at different gate biases shows different temperature dependences. From the aspect of the unique carrier behaviors of graded AlGaN/GaN heterostructure, we propose a quasi-multi-channel model to investigate the physics behind the temperature-dependent performance of AlGaN/GaN PolFETs.
文摘In this paper we study the gain saturation induced mode-coupling control in solid state ring laser devices based on the stimulated Raman effect of the polar crystals in.order to realize solid state ring laser gyroscopes. We theoretically investigate the mode coupling induced by gain saturation between clockwise (CW) and counterclockwise (CCW) propa- gating laser modes. Because the CW and CCW running waves are pumped with counter-propagating lasers respectively, the independent coexistence can be ensured.
基金supported by the National Key Technologies R&D Program,China(Grant No.2009ZX02302-002)the National Natural Science Foundation of China(Grant Nos.61376108,61076076,and 61076068)+2 种基金NSAF,China(Grant No.U1430106)the Science and Technology Commission of Shanghai Municipality,China(Grant No.13NM1400600)Zhuo Xue Plan in Hehai University,China
文摘Organic ferroelectric field-effect transistors (OFeFETs) are regarded as a promising technology for low-cost flexible memories. However, the electrical instability is still a critical obstacle, which limits the commercialization process. Based on already established models for polarization in ferroelectrics and charge transport in OFeFETs, simulation work is performed to determine the influence of polarization fatigue and ferroelectric switching transient on electrical characteristics in OFeFETs. The polarization fatigue results in the decrease of the on-state drain current and the memory window width and thus degrades the memory performance. The output measurements during the ferroelectric switching process show a hysteresis due to the instable polarization. In the on/off measurements, a large writing/erasing pulse frequency weakens the polarization modulation and thus results in a small separation between on- and off-state drain currents. According to the electrical properties of the ferroelectric layer, suggestions are given to obtain optimal electrical characterization for OFeFETs.
文摘The effects of the protic and aprotic polar solvents on the emission spectrum of the naphthalene-triethyl-amine system in THF were studied under conditions of steady-state illumination. The fluorescence spectrum of the naphthalene-triethylamine system consists of two emission bands, the fluorescence band of naphthalene(band A, 329 nm) and the emission band of the exciplex(band B, 468 nm). The intensities of both the emission bands decrease with increasing the solvent polarity. The intensity of band B also decreases due to the hydrogen-bonding interaction between triethylamine and protic solvent, while that of band A increases. It is thus suggested that the quenching of naphthalene fluorescence by triethylamine in THF occurs through the charge transfer and electron transfer reactions. The spectral changes upon the increase of solvent polarity can be explained by the dependences of the equilibrium constant between exciplex and ion-pair and the rate constant for the electron transfer reaction from triethylamine to the excited naphthalene on the relative permittivity of solvent. It is shown that the formation of intermolecular hydrogen-bonding between triethylamine and protic solvent suppresses the quenching reaction by the decrease in free amine. Acetonitrile has only a polar effect and trichloroacetic acid only a hydrogen-bonding(or protonation) effect, while alcohols have both the effects. The effects of alcohols could be separated into the effects of solvent polarity and intermolecular hydrogen-bonding interaction quantitatively.
基金Supported by the National Natural Science Foundation of China(No.10874096)
文摘To figure out the influence of isotope effect on product polarizations of the N(2D)+D2 reactive system and its isotope variants, quasi-classical trajectory(QCT) calculation was performed on Ho's potential energy surface(PES) of 2A″ state. Product polarizations such as product distributions of P(θr), P(φr) and P(θr,φr), as well as the generalized polarization-dependent differential cross sections(PDDCSs) were discussed and compared in detail among the four product channels of the title reactions. Both the intermolecular and intramolecular isotope effects were proved to be influential on product polarizations.
基金supported by the National Natural Science Foundationof China(6130214861101182)
文摘Target micromotion not only plays an important role in target recognition but also leads to esoteric characteristics in synthetic aperture radar (SAR) imaging. This paper finds out an interesting phenomenon, i.e. the angular extent effect, in micro-motion target images formulated by the polar format algorithm. A micromotion target takes on multiple pairs of paired echoes (PEs) around the true point, and each PE extends for an angle which is exactly equal to the angular extent of the synthetic aperture, regardless of the micromotion frequency. The effect is derived and interpreted by using the characteristics of Bessel functions. Then it is demonstrated by simulation experiments of a target with different micromotion frequencies. The revelation and interpretation of the effect is highly beneficial to micromotion-target SAR image understanding as wel as target recognition.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.91750104,11127403,and 11474130)the Natural Science Foundation of Jilin Province,China(Grant No.20160101332JC)
文摘We perform an experimental study of the multi-orbital effect on the high-order harmonic generation(HHG) from aligned N_2 molecules in both linearly and elliptically polarized intense laser fields.Measured by a home-built extreme ultraviolet(XUV) flat grating spectrometer with the pump-probe method, the angular distributions of different orders of HHG are obtained, which show distinctive behaviors for harmonics in the plateau and the cut-off regions.The ellipticity dependence of HHG is investigated by aligning the molecular axis parallel or perpendicular to the laser polarization.Our results indicate that both the highest occupied molecular orbital(HOMO) as well as the lower one(HOMO-1) contribute to the HHG of N2 molecules, in either linearly or elliptically polarized intense laser field.The study paves the way for understanding the ultrafast electron dynamics of molecules exposed to an intense laser field.
基金Project supported by Science Foundation of the Chongqing Committee of Education,China (Grant No KJ071205)
文摘A novel optimal design of sub-wavelength metal rectangular gratings for the polarizing beam splitter (PBS) is proposed. The method is based on effective medium theory and the method of designing single layer antireflection coating. The polarization performance of PBS is discussed by rigorous couple-wave analysis (RCWA) method at a wavelength of 1550 nm. The result shows that sub-wavelength metal rectangular grating is characterized by a high reflectivity, like metal films for TE polarization, and high transmissivity, like dielectric films for TM polarization. The optimal design accords well with the results simulated by RCWA method.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11127901,61521093,and 61505234)the International S&T Cooperation of Program of China(Grant No.2016YFE0119300)+1 种基金the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB160301)the Youth Innovation Promotion Association,Chinese Academy of Sciences
文摘The underlying mechanism of the spectral cleaning effect of the cross-polarized wave(XPW) generation process was theoretically investigated. This study shows that the spectral noise of an input spectrum can be removed in the XPW generation process and that the spectral cleaning effect depends on the characteristics of the input pulses, such as the chirp and Fourier-transform-limited duration of the initial pulse, and the modulation amplitude and frequency of the spectral noise. Though these factors codetermine the output spectrum of the XPW generation process, the spectral cleaning effect is mainly affected by the initial pulse chirp. The smoothing of the spectrum in the XPW generation process leads to a significant enhancement of the coherent contrast.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11547218,11564020,and 11504314)
文摘We investigate atomic above-threshold ionization in elliptically polarized strong laser fields with a semiclassical approach.With increasing laser intensity,the Coulomb focusing(CF) effects are found to become stronger in both parallel and perpendicular directions with respect to the polarization plane.The dependence of CF effects on tunnel exit,initial transverse momentum distribution and laser electric field is analyzed.It was revealed that the effects of tunnel exit are most prominent with variation of the laser intensity,and the other two factors both play non-negligible roles.Our results provide a deeper insight to the recent experiments of Coulomb asymmetry[Shafir D,et al.,2013 Phys.Rev.Lett.111 023005 and Li M,et al,2013 Phys.Rev.Lett.111 023006].
基金the National Natural Science Foundation of China under Grant (19575032)
文摘Analyzing powers and differential cross sections have been measured for elastic scattering of 22MeV polarized protons from 40Ca, 16O and 12C, and differential cross sections for inelastic scattering of 22 MeV protons from 3- (3.736 MeV) and 5-(4.491 MeV) states of 40Ca have also been measured. The experimental data for polarized proton elastic scattering have been analyzed with a phenomenological optical potential parameters, the experimental data and theoretical values are in good agreement. In the theoretical frame of microscopic single scattering model, transition densities extracted from electron inelastic scattering and M3Y and Halderson’s effective interactions have been utilized to analyze the experimental data of 22 MeV proton inelastic scattering from 40Ca. Overall, it seems that Halderson’s effective interaction can better describe the experimental data than M3Y although the degree of agreement between experimental and theoretical values needs to he improved.
基金Projected supported by the National Natural Science Foundation of China(Grant No.11174182)the Specialized Research Fund for the Doctoral Program of Higher Education,China(Grant No.20110131110005)
文摘By making use of the quasi-two-dimensional (quasi-2D) model, the current-voltage (l-V) characteristics of In0AsA10.82N/A1N/GaN heterostructure field-effect transistors (HFETs) with different gate lengths are simulated based on the measured capacitance-voltage (C-V) characteristics and I-V characteristics. By analyzing the variation of the electron mobility for the two-dimensional electron gas (2DEG) with electric field, it is found that the different polarization charge distributions generated by the different channel electric field distributions can result in different polarization Coulomb field scatterings. The difference between the electron mobilities primarily caused by the polarization Coulomb field scatterings can reach up to 1522.9 cm2/V.s for the prepared In0.38AI0.82N/A1N/GaN HFETs. In addition, when the 2DEG sheet density is modulated by the drain-source bias, the electron mobility presents a peak with the variation of the 2DEG sheet density, the gate length is smaller, and the 2DEG sheet density corresponding to the peak point is higher.