Climate change and air pollution are primarily caused by the combustion and utilization of fossil fuels.Both climate change and air pollution cause health problems.Based on the development of China,it is extremely imp...Climate change and air pollution are primarily caused by the combustion and utilization of fossil fuels.Both climate change and air pollution cause health problems.Based on the development of China,it is extremely important to explore the synergies of the energy transition,CO_(2) reduction,air pollution control,and health improvement under the target of carbon peaking before 2030 and carbon neutrality before 2060.This study introduces the policy evolution and research progress related to energy,climate change,and the environment in China and proposes a complete energy-climate-air-health mechanism framework.Based on the MESSAGE-GLOBIOM integrated assessment model,emission inventory and chemical transport model,and exposure-response function,a comprehensive assessment method of energy-climate-air-health synergies was established and applied to quantify the impacts of Chinese Energy Interconnection Carbon Neutrality(CEICN)scenario.The results demonstrate that,by 2060,the SO_(2),NO_(x) and PM_(2.5) emissions are estimated to be reduced by 91%,85%,and 90%respectively compared to the business-as-usual(BAU)scenario.The direct health impacts brought by achieving the goal of carbon neutrality will drive the proactive implementation of more emission reduction measures and bring greater benefits to human health.展开更多
Using N-methyl-D-glucosamine(NMDG)as the functional monomer,glycidyl methacrylate(GMA)as the connecting monomer,functionalized Fe3O4 nano-particles(NPs)as the support,three adsorbents were prepared including direct po...Using N-methyl-D-glucosamine(NMDG)as the functional monomer,glycidyl methacrylate(GMA)as the connecting monomer,functionalized Fe3O4 nano-particles(NPs)as the support,three adsorbents were prepared including direct polymer GMA-NMDG,magnetic GMA-NMDG polymer(MGN),and boron magnetic ion-imprinted polymer(BMIIP).Based upon the optimization of synthesis conditions,the prepared adsorbents and intermediate products were characterized using Fourier transform infrared spectroscopy,thermogravimetric analysis,scanning electron microscope,energy dispersive spectroscopy,X-ray diffraction,vibrating sample magnetometer,and Brunauer–Emmett–Teller to investigate the synthesis process,the morphological structure and the functional properties of the materials.The optimum performances of GMA-NMDG,MGN and BMIIP were obtained in the initial neutral solution(pH of 6.5).Moreover,GMANMDG and MGN reached the maximum adsorption capacity at 120 min,whereas BMIIP reached adsorption saturation at 60 min.The pseudo-second-order kinetic model was more suitable for the adsorption of boron using the adsorbents.The maximum adsorption capacity of GMA-NMDG was found to be 43.4 mg·g^(-1),while those of MGN and BMIIP were 32.5 and 28.3 mg·g^(-1),respectively.The Langmuir isotherm model was more appropriate to describe the adsorption process.The adsorbents maintained satisfactory adsorption performance within a certain temperature range.Competing ions had little effect on the adsorption of boron,and would be adsorbed simultaneously,due to which,the effect of co-adsorption can be considered.The adsorption capacity of GMA-NMDG was high,while the adsorption selectivity of BMIIP was much better.Furthermore,BMIIP showed good adsorption after five cycles of adsorption and desorption.The comparison of adsorbents showed that GMA-NMDG had the highest adsorption capacity and was suitable for co-adsorption.MGN had a high adsorption capacity,good comprehensive performance and magnetic properties.BMIIP had better adsorption rate,adsorption selectivity and recyclability.Through the optimization of synthesis conditions,the adsorption capacity of the traditional monomer NMDG polymer was increased,and the magnetism was given to facilitate rapid recovery.Combined with the ion imprinting technology,it showed higher boron adsorption selectivity in the presence of competitive ions.展开更多
We report the discovery of a peculiar X-ray transient,EP240408a,by Einstein Probe(EP)and follow-up studies made with EP,Swift,NICER,GROND,ATCA and other ground-based multiwavelength telescopes.The new transient was fi...We report the discovery of a peculiar X-ray transient,EP240408a,by Einstein Probe(EP)and follow-up studies made with EP,Swift,NICER,GROND,ATCA and other ground-based multiwavelength telescopes.The new transient was first detected with Wide-field X-ray Telescope(WXT)on board EP on April 8th,2024,manifested in an intense yet brief X-ray flare lasting for 12 s.The flare reached a peak flux of 3:9×10^(−9) erg cm^(−2) s^(−1) in 0.5-4 keV,∼300 times brighter than the underlying X-ray emission detected throughout the observation.Rapid and more precise follow-up observations by EP/FXT,Swift and NICER confirmed the finding of this new transient.Its X-ray spectrum is non-thermal in 0.5-10 keV,with a power-law photon index varying within 1.8-2.5.The X-ray light curve shows a plateau lasting for∼4 d,followed by a steep decay till becoming undetectable∼10 d after the initial detection.Based on its temporal property and constraints from previous EP observations,an unusual timescale in the range of 7-23 d is found for EP240408a,which is intermediate between the commonly found fast and long-term transients.No counterparts have been found in optical and near-infrared,with the earliest observation at 17 h after the initial X-ray detection,suggestive of intrinsically weak emission in these bands.We demonstrate that the remarkable properties of EP240408a are inconsistent with any of the transient types known so far,by comparison with,in particular,jetted tidal disruption events,gamma-ray bursts,X-ray binaries and fast blue optical transients.The nature of EP240408a thus remains an enigma.We suggest that EP240408a may represent a new type of transients with intermediate timescales of the order of∼10 d.The detection and follow-ups of more of such objects are essential for revealing their origin.展开更多
Climate change is one of the biggest health threats of the 21st century.Although China is the biggest developing country,with a large population and different climate types,its projections of large-scale heat-related ...Climate change is one of the biggest health threats of the 21st century.Although China is the biggest developing country,with a large population and different climate types,its projections of large-scale heat-related excess mortality remain understudied.In particular,the effects of climate change on aging populations have not been well studied,and may result in significantly underestimation of heat effects.In this study,we took four climate change scenarios of Tier-1 in CMIP6,which were combinations of Shared Socioeconomic Pathways(SSPs)and Representative Concentration Pathways(RCPs).We used the exposure-response functions derived from previous studies combined with baseline age-specific non-accidental mortality rates to project heat-related excess mortality.Then,we employed the Logarithmic Mean Divisia Index(LMDI)method to decompose the impacts of climate change,population growth,and aging on heat-related excess mortality.Finally,we multiplied the heat-related Years of Life Lost(YLL)with the Value of a Statistical Life Year(VSLY)to quantify the economic burden of premature mortality.We found that the heat-related excess mortality would be concentrated in central China and in the densely populated south-eastern coastal regions.When aging is considered,heat-related excess mortality will become 2.8–6.7 times than that without considering aging in 2081–2100 under different scenarios.The contribution analysis showed that the effect of aging on heat-related deaths would be much higher than that of climate change.Our findings highlighted that aging would lead to a severe increase of heat-related deaths and suggesting that regional-specific policies should be formulated in response to heat-related risks.展开更多
Egg yolk phospholipids(EPLs)are sensitive to oxidation and can produce large quantities of volatile compounds.This study monitored the oxidation process of EPLs at frying temperature.The changes in the classes of EPLs...Egg yolk phospholipids(EPLs)are sensitive to oxidation and can produce large quantities of volatile compounds.This study monitored the oxidation process of EPLs at frying temperature.The changes in the classes of EPLs,molar percentages of their fatty acyl groups and the concentrations of oxidation compounds under frying temperature were monitored by 31P nuclear magnetic resonance(NMR)and 1H NMR.Meanwhile,egg yolk triglycerides(ETGs)were used as controls.EPLs were mainly composed by phosphatidylcholine(76.74%±1.48%),phosphatidylethanolamine(17.97%±1.40%)and phosphatidylserine(1.26%±0.55%).EPLs,especially phosphatidylethanolamine,were degraded significantly during heating.The molar percentages of unsaturated acyl groups in EPLs were decreased,while the percentages of saturated plus modified acyl groups were increased during heating.EPLs produced large quantities of hydroperoxides and secondary oxidation compounds quickly.The results proved that EPLs were more sensitively to oxidation than ETGs during frying process,and EPLs could generate abundant of secondary oxidation compounds,especially 2,4-alkadienals,which demonstrated that EPLs are an ideal precursor of lipid-derived odorants.展开更多
In the last century,global pandemics have been primarily driven by respiratory infections,which consistently rank among the top 20 causes of death worldwide.The coronavirus disease 2019(COVID-19)pandemic has underscor...In the last century,global pandemics have been primarily driven by respiratory infections,which consistently rank among the top 20 causes of death worldwide.The coronavirus disease 2019(COVID-19)pandemic has underscored the intricate nature of managing multiple health crises simultaneously.In recent years,climate change has emerged as a major biosafety and population health challenge.Global warming and extreme weather events have intensified outbreaks of climate-sensitive infectious diseases,especially respiratory diseases.Influenza and COVID-19 have emerged as two of the most significant respiratory pandemics,each with unique epidemic characteristics and far-reaching consequences.Our comparative analysis reveals that while both diseases exhibit high transmission rates,COVID-19''s longer incubation period and higher severity have led to more profound and prolonged socioeconomic disruptions than influenza.Both pandemics have highlighted the exacerbating effects of climate change,with extreme weather events intensifying the spread and impact of these diseases.The COVID-19 pandemic exposed vulnerabilities in global healthcare systems and economies on an unprecedented scale,outstripping the strain caused by influenza outbreaks.Importantly,the COVID-19 pandemic has not only reshaped global public health strategies but also significantly impacted the epidemiology of influenza.Despite these differences and associations,both diseases underscore the urgent need for robust pandemic preparedness and adaptable public health strategies.This review delineates the overlaps and distinctions between influenza and COVID-19,offering insights into future challenges and the critical steps needed to enhance healthcare system resilience and improve global responses to pandemics.展开更多
基金supported by the GEIGC Science and Technology Project in the framework of“Research on Comprehensive Path Evaluation Methods and Practical Models for the Synergetic Development of Global Energy,Atmospheric Environment and Human Health”(grant No.20210302007).
文摘Climate change and air pollution are primarily caused by the combustion and utilization of fossil fuels.Both climate change and air pollution cause health problems.Based on the development of China,it is extremely important to explore the synergies of the energy transition,CO_(2) reduction,air pollution control,and health improvement under the target of carbon peaking before 2030 and carbon neutrality before 2060.This study introduces the policy evolution and research progress related to energy,climate change,and the environment in China and proposes a complete energy-climate-air-health mechanism framework.Based on the MESSAGE-GLOBIOM integrated assessment model,emission inventory and chemical transport model,and exposure-response function,a comprehensive assessment method of energy-climate-air-health synergies was established and applied to quantify the impacts of Chinese Energy Interconnection Carbon Neutrality(CEICN)scenario.The results demonstrate that,by 2060,the SO_(2),NO_(x) and PM_(2.5) emissions are estimated to be reduced by 91%,85%,and 90%respectively compared to the business-as-usual(BAU)scenario.The direct health impacts brought by achieving the goal of carbon neutrality will drive the proactive implementation of more emission reduction measures and bring greater benefits to human health.
基金supported by the National Natural Science Foundation of China(22078157)the Natural Science Foundation of the Jiangsu Higher Education institutions of China(21KJB610011)Postgraduate Research and Practice Innovation Program of Jiangsu Province(SJCX21_0468).
文摘Using N-methyl-D-glucosamine(NMDG)as the functional monomer,glycidyl methacrylate(GMA)as the connecting monomer,functionalized Fe3O4 nano-particles(NPs)as the support,three adsorbents were prepared including direct polymer GMA-NMDG,magnetic GMA-NMDG polymer(MGN),and boron magnetic ion-imprinted polymer(BMIIP).Based upon the optimization of synthesis conditions,the prepared adsorbents and intermediate products were characterized using Fourier transform infrared spectroscopy,thermogravimetric analysis,scanning electron microscope,energy dispersive spectroscopy,X-ray diffraction,vibrating sample magnetometer,and Brunauer–Emmett–Teller to investigate the synthesis process,the morphological structure and the functional properties of the materials.The optimum performances of GMA-NMDG,MGN and BMIIP were obtained in the initial neutral solution(pH of 6.5).Moreover,GMANMDG and MGN reached the maximum adsorption capacity at 120 min,whereas BMIIP reached adsorption saturation at 60 min.The pseudo-second-order kinetic model was more suitable for the adsorption of boron using the adsorbents.The maximum adsorption capacity of GMA-NMDG was found to be 43.4 mg·g^(-1),while those of MGN and BMIIP were 32.5 and 28.3 mg·g^(-1),respectively.The Langmuir isotherm model was more appropriate to describe the adsorption process.The adsorbents maintained satisfactory adsorption performance within a certain temperature range.Competing ions had little effect on the adsorption of boron,and would be adsorbed simultaneously,due to which,the effect of co-adsorption can be considered.The adsorption capacity of GMA-NMDG was high,while the adsorption selectivity of BMIIP was much better.Furthermore,BMIIP showed good adsorption after five cycles of adsorption and desorption.The comparison of adsorbents showed that GMA-NMDG had the highest adsorption capacity and was suitable for co-adsorption.MGN had a high adsorption capacity,good comprehensive performance and magnetic properties.BMIIP had better adsorption rate,adsorption selectivity and recyclability.Through the optimization of synthesis conditions,the adsorption capacity of the traditional monomer NMDG polymer was increased,and the magnetism was given to facilitate rapid recovery.Combined with the ion imprinting technology,it showed higher boron adsorption selectivity in the presence of competitive ions.
基金based on data obtained with Einstein Probe,a space mission supported by Strategic Priority Program on Space Science of Chinese Academy of Sciences,in collaboration with ESA,MPE and CNES(Grant No.XDA15310000)the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB0550200)+5 种基金the National Key R&D Program of China(Grant No.2022YFF0711500)the support by the National Natural Science Foundation of China(Grant Nos.12333004,12321003,12103065,12373040,12021003,12025303,12393814,and 12203071)the China Manned Space Project(Grant Nos.CMS-CSST-2021-A13,and CMS-CSST-2021-B11)the Youth Innovation Promotion Association of the Chinese Academy of Sciencessupported by a Ramón y Cajal fellowship(Grant No.RYC2021-030888-I)financial support from AGAUR,CSIC,MCIN and AEI 10.13039/501100011033(Grant Nos.PID2023-151307NB-I00,PIE 20215AT016,CEX2020-001058-M,and 2021-SGR-01270)。
文摘We report the discovery of a peculiar X-ray transient,EP240408a,by Einstein Probe(EP)and follow-up studies made with EP,Swift,NICER,GROND,ATCA and other ground-based multiwavelength telescopes.The new transient was first detected with Wide-field X-ray Telescope(WXT)on board EP on April 8th,2024,manifested in an intense yet brief X-ray flare lasting for 12 s.The flare reached a peak flux of 3:9×10^(−9) erg cm^(−2) s^(−1) in 0.5-4 keV,∼300 times brighter than the underlying X-ray emission detected throughout the observation.Rapid and more precise follow-up observations by EP/FXT,Swift and NICER confirmed the finding of this new transient.Its X-ray spectrum is non-thermal in 0.5-10 keV,with a power-law photon index varying within 1.8-2.5.The X-ray light curve shows a plateau lasting for∼4 d,followed by a steep decay till becoming undetectable∼10 d after the initial detection.Based on its temporal property and constraints from previous EP observations,an unusual timescale in the range of 7-23 d is found for EP240408a,which is intermediate between the commonly found fast and long-term transients.No counterparts have been found in optical and near-infrared,with the earliest observation at 17 h after the initial X-ray detection,suggestive of intrinsically weak emission in these bands.We demonstrate that the remarkable properties of EP240408a are inconsistent with any of the transient types known so far,by comparison with,in particular,jetted tidal disruption events,gamma-ray bursts,X-ray binaries and fast blue optical transients.The nature of EP240408a thus remains an enigma.We suggest that EP240408a may represent a new type of transients with intermediate timescales of the order of∼10 d.The detection and follow-ups of more of such objects are essential for revealing their origin.
基金supported by the National Natural Science Foundation of China(No.72091514)the Energy Foundation(No.G-2206-33982)+1 种基金the Tsinghua-Toyota Joint Research Fund,Wellcome Trust(No.209734/Z/17/Z)the GEIGC Science and Technology Project in the framework of the“Research on Comprehensive Path Evaluation Methods and Practical Models for the Synergetic Development of Global Energy,Atmospheric Environment and Human Health”(No.SGGEIG00JYJS2100056).
文摘Climate change is one of the biggest health threats of the 21st century.Although China is the biggest developing country,with a large population and different climate types,its projections of large-scale heat-related excess mortality remain understudied.In particular,the effects of climate change on aging populations have not been well studied,and may result in significantly underestimation of heat effects.In this study,we took four climate change scenarios of Tier-1 in CMIP6,which were combinations of Shared Socioeconomic Pathways(SSPs)and Representative Concentration Pathways(RCPs).We used the exposure-response functions derived from previous studies combined with baseline age-specific non-accidental mortality rates to project heat-related excess mortality.Then,we employed the Logarithmic Mean Divisia Index(LMDI)method to decompose the impacts of climate change,population growth,and aging on heat-related excess mortality.Finally,we multiplied the heat-related Years of Life Lost(YLL)with the Value of a Statistical Life Year(VSLY)to quantify the economic burden of premature mortality.We found that the heat-related excess mortality would be concentrated in central China and in the densely populated south-eastern coastal regions.When aging is considered,heat-related excess mortality will become 2.8–6.7 times than that without considering aging in 2081–2100 under different scenarios.The contribution analysis showed that the effect of aging on heat-related deaths would be much higher than that of climate change.Our findings highlighted that aging would lead to a severe increase of heat-related deaths and suggesting that regional-specific policies should be formulated in response to heat-related risks.
基金funded by National Natural Science Foundation of China(31960513).
文摘Egg yolk phospholipids(EPLs)are sensitive to oxidation and can produce large quantities of volatile compounds.This study monitored the oxidation process of EPLs at frying temperature.The changes in the classes of EPLs,molar percentages of their fatty acyl groups and the concentrations of oxidation compounds under frying temperature were monitored by 31P nuclear magnetic resonance(NMR)and 1H NMR.Meanwhile,egg yolk triglycerides(ETGs)were used as controls.EPLs were mainly composed by phosphatidylcholine(76.74%±1.48%),phosphatidylethanolamine(17.97%±1.40%)and phosphatidylserine(1.26%±0.55%).EPLs,especially phosphatidylethanolamine,were degraded significantly during heating.The molar percentages of unsaturated acyl groups in EPLs were decreased,while the percentages of saturated plus modified acyl groups were increased during heating.EPLs produced large quantities of hydroperoxides and secondary oxidation compounds quickly.The results proved that EPLs were more sensitively to oxidation than ETGs during frying process,and EPLs could generate abundant of secondary oxidation compounds,especially 2,4-alkadienals,which demonstrated that EPLs are an ideal precursor of lipid-derived odorants.
文摘In the last century,global pandemics have been primarily driven by respiratory infections,which consistently rank among the top 20 causes of death worldwide.The coronavirus disease 2019(COVID-19)pandemic has underscored the intricate nature of managing multiple health crises simultaneously.In recent years,climate change has emerged as a major biosafety and population health challenge.Global warming and extreme weather events have intensified outbreaks of climate-sensitive infectious diseases,especially respiratory diseases.Influenza and COVID-19 have emerged as two of the most significant respiratory pandemics,each with unique epidemic characteristics and far-reaching consequences.Our comparative analysis reveals that while both diseases exhibit high transmission rates,COVID-19''s longer incubation period and higher severity have led to more profound and prolonged socioeconomic disruptions than influenza.Both pandemics have highlighted the exacerbating effects of climate change,with extreme weather events intensifying the spread and impact of these diseases.The COVID-19 pandemic exposed vulnerabilities in global healthcare systems and economies on an unprecedented scale,outstripping the strain caused by influenza outbreaks.Importantly,the COVID-19 pandemic has not only reshaped global public health strategies but also significantly impacted the epidemiology of influenza.Despite these differences and associations,both diseases underscore the urgent need for robust pandemic preparedness and adaptable public health strategies.This review delineates the overlaps and distinctions between influenza and COVID-19,offering insights into future challenges and the critical steps needed to enhance healthcare system resilience and improve global responses to pandemics.
