The North Pacific storm track(NPST)is a high-frequency area of extratropical cyclones and an important channel for water vapor and energy transfer between low and mid–high latitudes.Previous weather and dynamic studi...The North Pacific storm track(NPST)is a high-frequency area of extratropical cyclones and an important channel for water vapor and energy transfer between low and mid–high latitudes.Previous weather and dynamic studies in this region have made significant progress,but due to the lack of ocean surface rainfall observation data,there is a lack of statistical research on precipitation in this area.In this study,statistical research on the spatiotemporal distribution characteristics of NPST rainfall was conducted based on GPM DPR(Global Precipitation Measurement Dual-frequency Precipitation Radar)observation data and ERA5 atmospheric parameters,and analysis and explanations are provided based on the atmospheric parameters.The study found that,compared to low-pressure systems,pressure gradients have a greater impact on cyclone activity and rainfall distribution.This feature,along with the meridional distribution of high atmospheric water vapor in the North Pacific Ocean and low in the north,collectively leads to the offset of high-frequency rainfall areas relative to storm tracks.The distribution of sea surface temperatures in the North Pacific Ocean affects the zonal distribution of storm tracks,causing weather disturbances and precipitation along the storm tracks to exhibit a northward extension from west to east.This study deepens our understanding of the role of NPST in global-scale water vapor and energy balance,and is of great significance for improving the prediction accuracy of climate models with respect to rainfall generated by extratropical cyclones.展开更多
Cathode materials that possess high output voltage,as well as those that can be mass-produced using facile techniques,are crucial for the advancement of aqueous zinc-ion battery(ZIBs)applications,Herein,we present for...Cathode materials that possess high output voltage,as well as those that can be mass-produced using facile techniques,are crucial for the advancement of aqueous zinc-ion battery(ZIBs)applications,Herein,we present for the first time a new porous K_(0.5)VOPO_(4)·1.5H_(2)O polyanionic cathode(P-KIVP)with high output voltage(above 1.2 V)that can be manufactured at room temperature using straightforward coprecipitation and etching techniques.The P-KVP cathode experiences anisotropic crystal plane expansion via a sequential solid-solution intercalation and phase co nversion pathway throughout the Zn^(2+)storage process,as confirmed by in-situ synchrotron X-ray diffraction and ex-situ X-ray photoelectron spectroscopy.Similar to other layered vanadium-based polyanionic materials,the P-KVP cathode experiences a progressive decline in voltage during the cycle,which is demonstrated to be caused by the irreversible conversion into amorphous VO_(x).By introducing a new electrolyte containing Zn(OTF)_(2) to a mixed triethyl phosphate and water solution,it is possible to impede this irreversible conversion and obtain a high output voltage and longer cycle life by forming a P-rich cathode electrolyte interface layer.As a proof-of-concept,the flexible fiber-shaped ZIBs based on modified electrolyte woven into a fabric watch band can power an electronic watch,highlighting the application potential of P-KVP cathode.展开更多
Histone H3 lysine 4 trimethylation(H3K4me3)is a canonical chromatin modification associated with active gene transcription,playing a pivotal role in regulating various cellular functions.Components of the H3K4me3 meth...Histone H3 lysine 4 trimethylation(H3K4me3)is a canonical chromatin modification associated with active gene transcription,playing a pivotal role in regulating various cellular functions.Components of the H3K4me3 methyltransferase complex,known as the proteins associated with SET1(COMPASS),have been implicated in exerting cancer-protective or cancer-inhibitory effects through inducive H3K4me3 modification.However,the role of the indispensable non-catalytic component of COMPASS CXXC-type zinc finger protein 1(CFP1)in malignant progression remains unclear.展开更多
基金funded by the National Natural Science Foundation of China(Grant Nos.42275140,42230612,91837310,41675041,and 92037000)the Second Tibetan Plateau Scientific Expedition and Research(STEP)program(Grant No.2019QZKK0104)。
文摘The North Pacific storm track(NPST)is a high-frequency area of extratropical cyclones and an important channel for water vapor and energy transfer between low and mid–high latitudes.Previous weather and dynamic studies in this region have made significant progress,but due to the lack of ocean surface rainfall observation data,there is a lack of statistical research on precipitation in this area.In this study,statistical research on the spatiotemporal distribution characteristics of NPST rainfall was conducted based on GPM DPR(Global Precipitation Measurement Dual-frequency Precipitation Radar)observation data and ERA5 atmospheric parameters,and analysis and explanations are provided based on the atmospheric parameters.The study found that,compared to low-pressure systems,pressure gradients have a greater impact on cyclone activity and rainfall distribution.This feature,along with the meridional distribution of high atmospheric water vapor in the North Pacific Ocean and low in the north,collectively leads to the offset of high-frequency rainfall areas relative to storm tracks.The distribution of sea surface temperatures in the North Pacific Ocean affects the zonal distribution of storm tracks,causing weather disturbances and precipitation along the storm tracks to exhibit a northward extension from west to east.This study deepens our understanding of the role of NPST in global-scale water vapor and energy balance,and is of great significance for improving the prediction accuracy of climate models with respect to rainfall generated by extratropical cyclones.
基金financially supported by National Natural Science Foundation of China(No.52102270)the Natural Science Foundation of Shandong Province of China(ZR2021QE002)+1 种基金the support from the Institute startup grant from Qingdao Universitythe Shandong Center for Engineered Nonwovens(SCEN)。
文摘Cathode materials that possess high output voltage,as well as those that can be mass-produced using facile techniques,are crucial for the advancement of aqueous zinc-ion battery(ZIBs)applications,Herein,we present for the first time a new porous K_(0.5)VOPO_(4)·1.5H_(2)O polyanionic cathode(P-KIVP)with high output voltage(above 1.2 V)that can be manufactured at room temperature using straightforward coprecipitation and etching techniques.The P-KVP cathode experiences anisotropic crystal plane expansion via a sequential solid-solution intercalation and phase co nversion pathway throughout the Zn^(2+)storage process,as confirmed by in-situ synchrotron X-ray diffraction and ex-situ X-ray photoelectron spectroscopy.Similar to other layered vanadium-based polyanionic materials,the P-KVP cathode experiences a progressive decline in voltage during the cycle,which is demonstrated to be caused by the irreversible conversion into amorphous VO_(x).By introducing a new electrolyte containing Zn(OTF)_(2) to a mixed triethyl phosphate and water solution,it is possible to impede this irreversible conversion and obtain a high output voltage and longer cycle life by forming a P-rich cathode electrolyte interface layer.As a proof-of-concept,the flexible fiber-shaped ZIBs based on modified electrolyte woven into a fabric watch band can power an electronic watch,highlighting the application potential of P-KVP cathode.
基金This work was supported by the National Key R&D Program of China(2021YFF1201303)the National Natural Science Foundation of China(81972196)+1 种基金the CAMS Innovation Fund for Medical Sciences(CIFMS)(2021-1-12M-012)the R&D Program of Beijing Municipal Education Commission(KJZD20191002302).
文摘Histone H3 lysine 4 trimethylation(H3K4me3)is a canonical chromatin modification associated with active gene transcription,playing a pivotal role in regulating various cellular functions.Components of the H3K4me3 methyltransferase complex,known as the proteins associated with SET1(COMPASS),have been implicated in exerting cancer-protective or cancer-inhibitory effects through inducive H3K4me3 modification.However,the role of the indispensable non-catalytic component of COMPASS CXXC-type zinc finger protein 1(CFP1)in malignant progression remains unclear.
